基于光电催化的硫化氢高值利用研究进展

doi:10.11896/cldb.22020097

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Abstract Hydrogen sulfide (H₂S) is a toxic gas widely generated in oil and gas fields and the petrochemical industry. The traditional Claus process not only consumes avast amount of energy but also does not reclaim the hydrogen energy stored in H₂S. Hence it is imminent to design new technology to achieve the high-value utilization of H₂S. Photoelectrocatalysis is a green and low-carbon technology that realizes the simultaneous conversion of H₂S into hydrogen energy and sulfur chemical products. However, the development of photoelectrocatalysts with high activity and poisoning resistance and value-added chemicals product obtained from the sulfur oxidation reaction are still tremendous challenges. Therefore, this review introduces the reaction principle, reaction types, photoelectrocatalyst design strategies, and H₂S coupling reaction systems. The research challenges and prospects associated with the photoelectrocatalytic splitting of H₂S are also provided, thus providing guidance to researchers in this field.

Key words： photoelectrocatalysis hydrogen sulfide hydrogen energy sulfur chemical product

Published: 10 February 2023 Online: 2023-02-23

CLC number:	O643.3
	O646

Fund:The National Natural Science Foundation of China (22178291, 22109132), the Provincial Key Research and Development Project of Sichuan (2022YFSY0052), and Scientific Research Starting Project of Southwest Petroleum University (2021QHZ014).

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	TANG Chun
	WU Mengnan
	DUAN Chao
	YU Tangjie
	YU Shan
	ZHOU Ying

Cite this article:

TANG Chun,WU Mengnan,DUAN Chao, et al. Research Progress of High-value Utilization of Hydrogen Sulfide Based on Photoelectrocatalysis[J]. Materials Reports, 2023, 37(3): 22020097-7.

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http://www.mater-rep.com/EN/10.11896/cldb.22020097 OR http://www.mater-rep.com/EN/Y2023/V37/I3/22020097

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