INORGANIC MATERIALS AND CERAMIC MATRIX COMPOSITES |
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Research Progress of High-value Utilization of Hydrogen Sulfide Based on Photoelectrocatalysis |
TANG Chun1,2,*, WU Mengnan2, DUAN Chao2, YU Tangjie2, YU Shan2, ZHOU Ying1,2,*
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1 State Key Laboratory of Oil and Gas Reservoir Geology and Exploitation, Southwest Petroleum University, Chengdu 610500, China 2 School of New Energy and Materials, Southwest Petroleum University, Chengdu 610500, China |
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Abstract Hydrogen sulfide (H2S) is a toxic gas widely generated in oil and gas fields and the petrochemical industry. The traditional Claus process not only consumes avast amount of energy but also does not reclaim the hydrogen energy stored in H2S. Hence it is imminent to design new technology to achieve the high-value utilization of H2S. Photoelectrocatalysis is a green and low-carbon technology that realizes the simultaneous conversion of H2S into hydrogen energy and sulfur chemical products. However, the development of photoelectrocatalysts with high activity and poisoning resistance and value-added chemicals product obtained from the sulfur oxidation reaction are still tremendous challenges. Therefore, this review introduces the reaction principle, reaction types, photoelectrocatalyst design strategies, and H2S coupling reaction systems. The research challenges and prospects associated with the photoelectrocatalytic splitting of H2S are also provided, thus providing guidance to researchers in this field.
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Published: 10 February 2023
Online: 2023-02-23
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Fund:The National Natural Science Foundation of China (22178291, 22109132), the Provincial Key Research and Development Project of Sichuan (2022YFSY0052), and Scientific Research Starting Project of Southwest Petroleum University (2021QHZ014). |
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