g-C<sub>3</sub>N<sub>4</sub>/过渡金属硫化物复合材料的结构设计、合成及光催化应用

doi:10.11896/cldb.20100135

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Abstract Graphite carbonnitride (g-C₃N₄), as an inorganic non-metallic semiconductor photocatalytic material, comprises a special energy band and crystal structure, which receives extensive attention in environmental governance and clean energy. However, the single-phase g-C₃N₄ has disadvantages of small response range to natural light, small specific surface area, few reactive sites, and high recombine efficiency of photoelectron-hole pairs, which limit its large-scale utilization in the field of photocatalysis. Transition metal sulfides have a special energy band structure, and excellent physical and photocatalytic properties, which show great development potential in photocatalytic applications. There were numerous researches generally focused on the construction of heterojunctions to solve the problems that catalytic materials has, such as narrow optical response range, low photocatalytic quantum efficiency due to the easy combination of carriers, short duration of carriers and insufficient reactive sites. Herein, the performance, structure design and reaction mechanism of the g-C₃N₄/transition metal sulfide photocatalytic materials were reviewed, the progress of the heterogeneous junction construction was discussed, and the development prospect of the g-C₃N₄/transition metal sulfide composite materials was prospected.

Key words： catalytic material photocatalysis photochemistry nanomaterial g-C₃N₄ transition metal sulfide

Published: 10 January 2023 Online: 2023-01-31

CLC number:

TB333

Fund:Natural Science Foundation of Jiangsu Province (BK20180103,BK20180971),Natural Science Foundation of Universities in Jiangsu Province(16KJA430008),Funding Project of Advantageous Discipline Construction Project for Universities in Jiangsu Province, Suzhou Science and Technology Development Plan Project (SYG201742,SYG201818,SS202036),Suzhou Weina Key Laboratory of Optoelectronic Materials and Sensors(SZS201812),and Jiangsu Graduate Practice Innovation Program(SJCX20_1107).

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	TANG Fei
	CAI Wenyu
	CHEN Fei
	ZHU Chen
	LIU Chengbao
	CHEN Zhigang

Cite this article:

TANG Fei,CAI Wenyu,CHEN Fei, et al. Structural Design, Synthesis and Photocatalytic Applications of g-C₃N₄/Transition Metal Sulfide Composite Material[J]. Materials Reports, 2023, 37(1): 20100135-9.

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http://www.mater-rep.com/EN/10.11896/cldb.20100135 OR http://www.mater-rep.com/EN/Y2023/V37/I1/20100135

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