| INORGANIC MATERIALS AND CERAMIC MATRIX COMPOSITES |
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| Recent Advancement of Novel Composites Based on Two-dimensional MXene-supported Nano-metals and Its Oxides |
| LI Hui1, ZHU Gang1,*, ZHANG Jianwei2, KANG Kunyong1, DU Guanben3, LI Yuanyuan1, SUN Ke1
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1 College of Material Science and Engineering, Southwest Forestry University, Kunming 650224, China
2 College of Physics Science and Engineering, Tongji University, Shanghai 200092, China
3 Key Laboratory for Forest Resource Conservation and Utilization in the Southwest Mountains of China, Southwest Forestry University, Kunming 650224, China |
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Abstract MXene is a novel unique type of two-dimensional layered graphene-liked structural, which exhibits exceptional optical, electrical properties and thermodynamic properties, with large specific surface area, superior hydrophilicity and abundant controllable surface functional groups, as a novel carrier of nano-metals and its oxides, it provides favorable conditions for the microstructure enhancement design of nanocomposites to give better exert the interfacial effects.However, 2D MXene suffers from the difficulties of easy autonomous stacking of lamellae, difficulty in precisely regulating the geometric distribution and composite conformation of nano metals and their oxides in MXene carriers, and weak interfacial bonding of the composites, which leads to the failure to maximize the synergy, coupling and multifunctional response mechanisms between diffe-rent components. Especially for 2D MXene nano-carrier with significant intrinsic functional properties (including thermal and electrical conductivity and mechanical properties), its excellent properties are difficult to fully reflect, which significantly affects the comprehensive properties of the composites. For the above-mentioned issues, preliminary exploration has been carried out on construction of high-performance composites based on 2D MXene-supported nano-metals and their oxides in China and abroad. The related research results have already been applied practically to energy storage, photocatalysis, electromagnetic shielding, microwave absorption, supercapacitors and other frontier fields, and some impressive strides and progress have been made. Hence, this review paper presents the main preparation methods, microstructure and functional properties of 2D MXene supported metal and its oxide nanocomposites. The application and the enhanced mechanism in energy storage, microwave absorption, etc. are summarized. Moreover, some challenges are pointed out, and the future directions of research in this field and their application prospects are forecasted. It is expected to provide a solid theoretical and experimental foundation for the microstructure regulation and perfor-mance optimization design of the novel MXene-based nanocomposites.
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Published: 10 May 2022
Online: 2022-05-09
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| Fund:Natural Science Foundation of Yunnan Province, China (2017FB144). |
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2022, Vol. 36 
