INORGANIC MATERIALS AND CERAMIC MATRIX COMPOSITES |
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Recent Progress in MOFs-based Sulfur Cathode for Li-S Batteries |
WEI Anke, WANG Lei*, WANG Yi
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College of Materials Science and Engineering, Xi'an Shiyou University, Xi'an 710065, China |
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Abstract With the development of portable electronic devices and electric vehicles, the widely used lithium ion batteries can no longer satisfy the market demand. Lithium sulfur batteries, as a promising high-energy chemical power source, have attracted extensive attention of researchers due to their high theoretical specific capacity (1 675 mAh·g-1) and high theoretical energy density (2 600 Wh·kg-1). However, some of the challenges in the development of lithium-sulfur batteries are inevitable, including the low conductivity of sulfur, large volume changes before and after charge and discharge, poor cycle stability, and the easy dissolution of polysulfide generated. It has been demonstrated that combining sulfur with MOFs-based materials with different structures to build composite cathode materials with a unique microstructure can significantly improve the conductivity, cyclic stability and the dissolution of polysulfide. In this review, the advantages of MOFs as sulfur carriers and recent research progress in MOFs-based sulfur cathode materials are summarized and commented upon based on the principle of lithium-sulfur batteries. Meanwhile, it also gives brief suggestions and outlooks on the future research directions in lithium-sulfur batteries.
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Published: 14 July 2021
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Fund:This work was financially supported by the National Natural Science Foundation Youth Fund of China (51702257), Natural Science Basic Research Plan in Shaanxi Province of China (2018JQ5123), Provincial Superiority Discipline of Materials Science and Engineering of Xi’an Shiyou University (ys37020203). |
About author:: Anke Wei, received his B.S. degree in applied chemistry from Yan’an University in 2018. He is currently pursuing his master degree at the College of Materials Science and Engineering, Xi’an Shiyou University under the supervision of Mr. Wang. His research has focused on the application of metal organic framework in lithium ion battery.
Lei Wang, received his Ph.D. degree in materials from Shandong University in 2014. He is currently an associate professor in School of Materials Science and Engineering of Xi’an Shiyou University. His research interests are design and preparation of functional crystal materials, material simulation and calculation. |
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