纳米粒子自组装超结构的制备及基于构效关系的性能

doi:10.11896/cldb.21120161

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Abstract With the mature control of morphology and size of nanoparticles, the superstructure can be self-assembled with regular lattice structure from highly monodispersed nanoparticles (size deviation ≤5%). Nanomaterials scientists use the concept of ‘artificial solids’ to construct self-assembled superstructures, by exploiting nanoparticles as ‘artificial atoms’ in building supercrystals with different stacking modes through interactions between the adjacent particles. As a ‘bottom-up’ fabrication approach, the self-assembly method can achieve fabrication of material devices in large area. Structure-activity relationship is a basic principle that widely exists in nature. It refers to the relationship between the composition and structure of a substance and its physical and chemical properties. The self-assembled superstructures of nanoparticles based on different constructed bricks and stacking modes show special collective properties different fromboth individual nanoparticles and their bulk materials, and show broad application prospects in optics, electricity, catalysis, biomedicine and other fields. Based on the interaction between nanoparticles and taking full advantage of the external environment, researchers have developed a series of self-assembly methods to construct superstructures with customized performance, which is realized by designing the building blocks and stacking structures from the point of view of desired material properties.
This review offers a retrospection of the self-assembled mechanism, methods, and research progress in this area, and provides elaborate descriptions about how the assembled superstructures take effects on their optical, electric, magnetic, and mechanical properties. It is focused on the embodiment of properties arising from the structure-activity principle in the self-assembled superstructures. By changing the components and structures of the self-assembled nanoparticles superstructures, different physical and chemical properties can be obtained to adapt to different application fields.

Key words： nanoparticle self-assembly superstructure structure-activity collective property

Published: 10 September 2023 Online: 2023-09-05

CLC number:

O648

Fund:National Natural Science Foundation of China (21904120, 62073299, 51902344), Henan Province Science and Technology Programs (212102310858), Project of Central Plains Science and Technology Innovation Leading Talents (224200510026), Ph.D. Start-up Fund of Zhengzhou University of Light Industry (2018BSJJ022).

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	QIN Xiaoyun
	SHAO Wenlong
	TIAN Kuan
	JIANG Liying
	LUO Dan

Cite this article:

QIN Xiaoyun,SHAO Wenlong,TIAN Kuan, et al. Preparation of Self-assembled Nanoparticles Superstructures and Their Properties Based on Structure-Activity Principle[J]. Materials Reports, 2023, 37(17): 21120161-12.

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http://www.mater-rep.com/EN/10.11896/cldb.21120161 OR http://www.mater-rep.com/EN/Y2023/V37/I17/21120161

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