铁含量对Fe-P-C非晶合金降解亚甲基蓝性能的影响

doi:10.11896/cldb.21060276

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Abstract In this work, four kinds of Fe_80+2xP_10-xC_10-x(x=0,1,2,3, at%) amorphous alloy ribbons with different Fe contents were prepared. The catalytic degradation of methylene blue (MB) solution by Fe_80+2xP_10-xC_10-x(x=0,1,2,3, at%) amorphous alloy ribbons was studied by Fenton-like reaction. The results show that Fe-P-C amorphous alloy ribbons exhibit excellent degradation performance of MB solution by Fenton-like reaction, and the higher the iron content, the better the degradation performance. However, when the iron content exceeds 82at%, the effect of iron content on the degradation performance is not obvious.The surface morphology observation showed that with the increase of Fe content, the surface of the Fe-P-C amorphous ribbon after reaction showed a more porous structure, which was beneficial to obtain high degradation efficiency. The cyclic degradation test shows that the four Fe-P-C amorphous alloys with different iron contents have little difference and have long service life, which may be related to the formation of surface morphology with loose lamellar structure and 3D flower-like grid structure during the degradation process. The results of X-ray electron energy spectrum analysis showed that the different Fe content did not affect the degradation reaction mechanism of Fe-P-C amorphous alloy.

Key words： Fe-based amorphous alloys Fenton-like reaction methylene blue(MB) degradation

Published: 30 November 2021

CLC number:

TG139+.8

Fund:National Natural Science Foundation of China (51771161).

About author:: Yaya Ma received her M.S. degrees in June 2021 from Xinjiang University. During the postgraduate period, she was mainly engaged in the research of the catalytic performance of iron-based amorphous alloys.
Qiang Li, professor, doctoral supervisor of Xinjiang University, enjoying the special government allowance of the State Council. He obtained his Ph. D. degree from the Chinese University of Hong Kong in 2002. He has worked in the School of Physical Science and Technology at Xinjiang University since 2005, and his main research directions include alloy transformation, bulk amorphous alloys and amorphous alloy coatings. So far, he has been granted 5 projects from the National Natural Science Foundation of China as the chief investigator and published more than 60 SCI papers in academic journals.

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Cite this article:

MA Yaya,LI Qiang,MU Baoxia, et al. Effect of Iron Content on the Degradation of Methylene Blue in Fe-P-C Amorphous Alloy[J]. Materials Reports, 2021, 35(21): 21085-21090.

URL:

http://www.mater-rep.com/EN/10.11896/cldb.21060276 OR http://www.mater-rep.com/EN/Y2021/V35/I21/21085

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