基于水泥基材料的CO<sub>2</sub>矿化封存利用技术综述

doi:10.11896/cldb.20100295

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Abstract In order to mitigate the negative impact of CO₂ emissions from cement production on the global climate change, CO₂ was sequestered in cement-based materials in the form of inorganic carbonate by utilizing the mineralization reaction between CO₂ and cementitious materials containing Ca²⁺ and Mg²⁺ and their hydration products based on carbon capture, storage and utilization (CCUS) technology. Meanwhile, due to the good stability, filling effect and nucleation effect of its mineralized products (mainly calcium carbonate and amorphous SiO₂), the mechanical properties and durability of cement-based materials after CO₂ mineralization were effectively improved, and the cement-based materials with high performance were obtained in a short time. This paper reviews currently primary methodologies for the mineralization of CO₂ in cement-based material. First, we discuss the reaction characteristics of different cementitious materials and CO₂ in the maintenance process of concrete. Second is property improvement of recycled concrete aggregate by mineral carbonation. The CO₂ mineralization and utilization technology to improve the mechanical performance of concrete and the quality of recycled concrete aggregate in detail in the perspectives of micro-mechanisms, factors influencing reaction kinetics and CO₂ absorption are introduced emphatically. Finally, based on current research status and existing problems, the future development and research direction for CO₂ mineralization of cement-based material are also proposed.

Key words： carbon capture utilization and storage (CCUS) mineral carbonation cement-based material CO₂-curing recycled concrete aggregate

Published: 10 October 2022 Online: 2022-10-12

CLC number:

X701

Fund:National Natural Science Foundation of China (51604288), the Open Project of the State Key Laboratory of Green Building Materials(2019GBM10), and the Key Laboratory of Road Construction Technology and Equipment (300102250505)

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	LI Linkun
	LIU Qi
	HUANG Tianyong
	LI Yang
	PENG Bo

Cite this article:

LI Linkun,LIU Qi,HUANG Tianyong, et al. Review on CO₂ Mineralization, Sequestration and Utilization of Cement-based Materials[J]. Materials Reports, 2022, 36(19): 20100295-9.

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http://www.mater-rep.com/EN/10.11896/cldb.20100295 OR http://www.mater-rep.com/EN/Y2022/V36/I19/20100295

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