METALS AND METAL MATRIX COMPOSITES |
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Research Progress of Oxygen Reduction Catalysts Based on Metal-Organic Framework Materials |
REN Yufeng, LUAN Weiling, JIANG Tao
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Key Laboratory of Pressure Systems and Safety (MOE), School of Mechanical and Power Engineering, East China University of Science and Technology, Shanghai 200237, China |
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Abstract With the advantages of high power generation efficiency, low pollution and noise, and reliable operation, fuel cells have attracted widespread attention from various countries as they can be used as the main power source for new energy vehicles. Oxygen reduction reaction (ORR), as an important electrochemical reaction in fuel cells, has higher requirements on catalysts. However, the high cost and low durability of Pt catalyst used widely restrict the development of new energy vehicles. Non-Pt catalysts or low-Pt catalysts can reduce costs while maintaining the same performance, which is the key to promoting the commercial application of fuel cell vehicles. Metal-free catalysts and transition metal catalysts prepared by metal-organic framework materials (MOF) can completely replace precious metal Pt catalysts. Among them, the Fe-based and Co-based MOF catalysts developed using the ZIF series are the focus of ORR research. In addition, inspired by non-precious metal catalysts, low-Pt catalysts are supported or alloyed through MOF, which further improves low-Pt catalysts electrochemical activity and durability. This paper reviews the recent research progress of ORR catalysts based on MOF materials, introduces the research status and challenges of metal-free catalysts, transition metal catalysts and precious metal catalysts, and provides technical support for obtaining ORR catalysts with superior performance.
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Published: 10 October 2022
Online: 2022-10-12
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Fund:National Natural Science Foundation of China (51475166), and Shanghai Automobile Industry Science and Technology Development Foundation (1801) |
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