| MATERIAL .S AND SUSTAINABL E DEVEL OPMENT: MATERIAL .S REMANUFACTURING AND WASTE RECYCLING |
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| Research Progress on Setting and Hardening of Geopolymers and Their Control |
| WANG Aiguo1, WANG Xingyao1, SUN Daosheng1,*, ZHU Yingcan2, LIU Kaiwei1, JING Yan1, GUAN Yanmei1
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1 Anhui Key Laboratory of Advanced Building Materials, Anhui Jianzhu University, Hefei 230022, China
2 University of Southern Queensland, Centre for Sustainable Agricultural Systems, Toowoomba, QLD 4350, Australia |
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Abstract Geopolymers are a family of non-traditional cementitious materials formed by alkali-activation of reactive aluminosilicate minerals, which have the characteristics of high strength, good durability, green and environmental friendly. However, the diversity of raw materials and alkaline activators bring about the complexity of hydration (activation) mechanisms, and lead to the uncertainty of setting and hardening process. In addition, the change of temperature during manufacturing also has a great impact. Depending on the raw materials and preparation conditions, the setting and hardening of geopolymers may go to two extremes: on one hand, too rapid setting and accelerated hardening to work with, on the other hand, too slow to gain early strength. Therefore, control the setting time of geopolymers within a reasonable range is one of the key issues that address the problems of application. Based on the calcium-rich, low-calcium, calcium-free categories of geopolymer systems, this article clarified the setting and hardening mechanism of geopolymers, analyzed the influence of fineness, activity and CaO content of aluminosilicate materials, types and dosage of alkaline activators, as well as temperature on the setting time of geopolymers. It summarized the technical methods to regulate the setting time of geopolymers and analyzed its mechanism. It is expected to provide technical support for the application research of geopolymers.
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Published: 14 July 2021
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| Fund:This work was financially supported by the National Natural Science Foundation of China (51778003), Key Research and Development Projects in Anhui Province (202004611020033) and Natural Science Foundation of Anhui Provincial Education Department (KJ2019JD16). |
About author:: Aiguo Wang received his Ph.D. degree in materials from Nanjing Tech University in 2010. He performed his visiting researches in University of Southern Queen-sland, Centre for Future Materials of Australia in 2017. He has been a master tutor from 2013 in Anhui Jianzhu University. He was granted professor in 2019. He has hosted 10 provincial or ministerial level research projects including National Natural Science Foundation of China, Natural Science Foundation of Higher Education of Anhui Province, Open Project of State Key Laboratory of High Perfor-mance Civil Engineering Materials, and Open Project of State Key Laboratory of Materials and Chemical Engineering, and so on. He assumes reviewer of journals like Construction and Building Materials, Cement and Concrete Composites, Cement and Concrete Composites, Materials Review, Bulletin of the Chinese Ceramic Society. He is also the director of Building Materials Branch of China Architectural Society. His major interests are high perfor-mances cementitious composite materials, building functional materials & comprehensive utilization of solid waste.
Daosheng Sun received his B.E. degree in building materials and products from Chongqing University in 1986 and received his Ph.D. degree in materials from the Nanjing Tech University in 2004. He was granted professor in 2005. He is the tutor of Anhui Jianzhu University and Hefei Institute of Physical Science,Chinese Academy of Sciences. He is the member of Anhui Silicate Society, Anhui Cement Standardization Technical Committee and Anhui Cement Association. His research interests include high-performance concrete, comprehensive utilization of solid waste, and advanced building materials. |
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2021, Vol. 35 
