三维、二维卤化物钙钛矿材料性能及应用综述

doi:10.11896/cldb.20070246

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Abstract Halide perovskite materials are currently a research hot spot in academia, but there are few comparative analyses of the properties of two-dimensional (2D) and three-dimensional (3D) halide perovskite materials. Through comparison, this article summarizes the different physical and chemical properties of the materials after the dimensional change and the reasons for the property change, and the application fields and problems faced by different properties are analyzed, which provides ideas for the future research of perovskite materials.
First of all, both 3D and 2D halide perovskites have the characteristics of adjustable band gap and high tolerance to defects, but the 2D material is more stable than the 3D material in terms of structural stability. The reason is that the 2D halide perovskite material has low combination energy and high tolerance to deformation. Secondly, since the 3D halide perovskite material is dimensionally reduced to obtain a 2D halide perovskite, the periodic metal framework is destroyed during the process. Some electron donor defects or hole acceptor defects have deep energy levels in the 2D material, resulting in the decrease of carrier concentration and the decrease of electronic transmission performance. The 2D material has poor electric mobility ability compared with the 3D material. At the same time, the quantum effect of the 2D material is prominent and the light absorption ability is reduced, so three-dimensional halide perovskites are more suitable for use in solar cell light absorption layers than two-dimensional materials. Thirdly, on the one hand, the 3D halide perovskite materials currently used in light-emitting devices have low external quantum efficiency and require the introduction of work function-matched semiconductor materials to form heterostructures in order to be efficiently applied. On the other hand, although 2D halide perovskites can achieve a variety of continuous luminous spectrum, but the processing technology needs to be improved to meet the needs of large-scale commercial production. Finally, traditional perovskites, as lead-containing compounds, decomposition will affect the environment, so we should produce the new lead-free stable halide perovskite.

Key words： perovskite materials dimension-change structural comparison properties and applications

Published: 10 March 2022 Online: 2022-03-08

CLC number:

O649.4

Fund:National Natural Science Foundation of China (12064027, 11804058, 62065014, 11264031),the Aeronautical Science Foundation of China (2017ZC56003), the Open Fund of Jiangxi Key Laboratory of Image Processing and Pattern Recognition (ET201908119), the Special Fund of Nanchang Hangkong University Graduate, China (YC2020073), the Open Fund of the Key Laboratory of Nondestructive Testing of Ministry of Education, China (EW201908442, EW201980090), Natural Science Foundation of Jiangxi Province (20192BAB202006, 20192BAB207001,20151BAB207054), and Science and Technology Project of Jiangxi Education Department (GJJ170594).

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	SONG Lingting
	XIAO Wenbo
	HUANG Le
	WU Huaming

Cite this article:

SONG Lingting,XIAO Wenbo,HUANG Le, et al. A Review of Three-dimensional and Two-dimensional Halide Perovskite Materials in Their Properties and Applications[J]. Materials Reports, 2022, 36(5): 20070246-7.

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http://www.mater-rep.com/EN/10.11896/cldb.20070246 OR http://www.mater-rep.com/EN/Y2022/V36/I5/20070246

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