基于天然贻贝仿生制备聚多巴胺改性石墨烯基功能材料及其水体环境修复应用研究进展

doi:10.11896/cldb.19030036

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Abstract The global water pollution problem is becoming increasingly serious. Graphene can be a good choice for designing and fabricating various graphene-based functional materials due to its large specific surface area and excellent decontamination performance. However, graphene sheets readily aggregate and agglomerate themselves, causing a loss of their fabulous properties. It is therefore necessary to modify the surface of graphene to make it dispersible in various water media. Inspired from naturally occurring mussel and its excreted adhesive protein, the chemical modifications of graphene can thus be efficiently achieved based on such a natural way. The resulting polydopamine (Pdop)-modified graphene (Pdop-G) exhibits excellent dispersibility, facilitating its further manufacturing through facile solution-based routes. Such modification also enables the generation of more active sites for diverse applications, and a versatile platform can be provided as well due to the modification. As a consequence, Pdop-G has captured the focus of much attention for various applications, especially environmental remediation.
This paper reviews the design and preparation methods of Pdop-G and related materials over the past three years, and special attention is placed on the research status in environmental remediation applications using a diversity of Pdop-G-based functional materials, mainly including three critical strategies (i.e., adsorption, membrane filtration and photocatalysis). This literature review shows that Pdop-G and related materials have great application potential in dealing with water contaminants, but it is necessary to improve the preparation and manufacturing processes, post-treatment strategies, and other conditions to achieve commercial applications. This review paper sufficiently comments on the merits and demerits of using graphene chemistry, mussel-inspired biomimetic chemistry, and the corresponding technologies for environmental remediation applications, and also suggests the research directions on which future efforts can be put, in order to clarify the scope of applications and the routes to developing technologies. We hope this review paper can provide a guide for researchers when concerning the bio-inspired modification of graphene and the resulting modified graphene-based functional materials for various applications, especially environmental remediation. It is also highly expected that innovative ideas and new research directions will be obtained as a result of this review contribution.

Key words： polydopamine graphene adsorption membrane filtration photocatalysis environmental remediation

Published: 13 May 2020

CLC number:

TQ042

Fund:This work was financially supported by the National Natural Science Foundation of China (51702050), the Featured Innovation Project of the Department of Education of Guangdong Province (2017KTSCX188), the Open Research Foundation of Guangdong Provincial Key Laboratory of New and Renewable Energy Research and Development (Y807s31001), the Open Research Foundation of Guangdong Provincial Key Laboratory of Industrial Surfactant (GDLS-01-2019), and Specially-Appointed Professor program of Foshan University.

About author:: Huawen Hu received his Ph.D. degree in materials scie-nce from the Hong Kong Polytechnic University (China) in 2015. After continuing one-year postdocto-ral research at the Hong Kong Polytechnic University (China), he joined the faculty of the School of Mate-rials Science and Energy Engineering (Foshan University) in 2016. He was elected to the Top-notch Young Talents Program of Pearl River Recruitment Program of Talents in 2018. He has published more than 60 scientific papers, and is currently an associate professor and postgraduate supervisor. His research inte-rests are low-dimensional functional materials for energy, catalysis, sensing and environmental remediation applications.

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	ZHU Wuqing
	QUAN Haiyan
	PENG Shusen
	ZHANG Min
	CHEN Dongchu
	HU Huawen

Cite this article:

ZHU Wuqing,QUAN Haiyan,PENG Shusen, et al. Recent Advances in Mussel-inspired Polydopamine-modified Graphene-based Functional Materials and Their Applications in Waterborne Environmental Remediation[J]. Materials Reports, 2020, 34(11): 11009-11021.

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http://www.mater-rep.com/EN/10.11896/cldb.19030036 OR http://www.mater-rep.com/EN/Y2020/V34/I11/11009

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