| INORGANIC MATERIALS AND CERAMIC MATRIX COMPOSITES |
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| Research Progress of High Crystallinity g-C3N4 in Photocatalysis |
| XU Yang1,2, LIU Chengbao1,2,3,*, ZHENG Leizhi1,2,3, CHEN Feng1,2,3, QIAN Junchao1,2,3, QIU Yongbin4, MENG Xianrong5, CHEN Zhigang1,2,3
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1 Jiangsu Key Laboratory for Environment Functional Materials, Suzhou University of Science and Technology, Suzhou 215009, Jiangsu, China
2 School of Materials Science and Engineering, Suzhou University of Science and Technology, Suzhou 215009, Jiangsu, China
3 Jiangsu Collaborative Innovation Center of Technology and Material for Water Treatment, Suzhou University of Science and Technology, Suzhou 215009, Jiangsu, China
4 Jiangsu Province Ceramics Research Institute Co., Ltd.,Yixing 214221, Jiangsu, China
5 Suzhou Institute of Environmental Science, Suzhou 215007, Jiangsu, China |
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Abstract Graphite phase carbon nitride (g-C3N4), a polymer semiconductor with a typical two-dimensional layered structure and narrow band gap, has excellent visible light absorption capacity, stable physical and chemical properties and good photocatalytic properties. However, the structure of g-C3N4 produced by the heat-induced polymerization from traditional nitrogen-containing precursor is incomplete. The main body is melon-based carbon nitride with amorphous or semi-crystalline structure. There are many defects in its phase and surface, which lead to lower conductivity, higher electron-hole pairs recombination rate, resulting in lower catalytic activity. Therefore, it is necessary to improve the crystallinity of g-C3N4. This paper mainly summarizes the advantages of high crystalline carbon nitride (CCN) and the research progress in recent years. Increasing the crystallinity of g-C3N4 can provide charge transfer channels between the conjugated planes to improve the charge transfer efficiency, and also introduce other modification methods to achieve efficient synergies. Then, the structure, characterization, preparation, modification strategy and application fields of CCN in recent years were reviewed. Finally, the challenges and future development directions of CCN photocatalysts are summarized briefly.
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Published: 10 November 2024
Online: 2024-11-11
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| Fund:Natural Science Foundation of Jiangsu Province (BK20180103,BK20180971), Suzhou Science and Technology Deve-lopment Plan Project (SS202036). |
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2024, Vol. 38 
