二维碳基材料在锂硫电池中的研究进展

doi:10.11896/cldb.23100229

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Abstract Lithium-sulfur batteries (Li-S batteries) are regarded as one of the most promising modern energy storage systems due to their high theoretical energy density and specific capacity. However, their commercial application still faces huge challenges, such as fast capacity decay, poor cycle stability and short lifetime, originating from the shuttle effect, high electrochemical energy barrier, low conductivity of sulfur species, and volume change of sulfur cathode. Optimizing functional separators and designing appropriate positive electrode materials for batteries is a feasible approach. Two-dimensional (2D) carbon-based materials are now widely used in Li-S batteries as sulfur host materials, since they are highly controllable and have a wide range of physical, chemical, and electrochemical characteristics. This paper reviews the research progress of 2D carbon-based materials in Li-S batteries, including graphene, 2D defective carbon-based materials, non-metallic doped carbon-based materials, metal-doped carbon-based materials, non-metallic carbides and metal carbides, and their corresponding catalytic performance. Finally, we highlight a few issues that still require addressing and forecast the future development in the application of Li-S batteries.

Key words： lithium-sulfur battery two-dimensional carbon-based material shuttle effect conductivity modification

Published: 10 April 2025 Online: 2025-04-10

CLC number:

O4-1

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	Articles by authors
	XU Wanlin
	FENG Tengrui
	WU Qi
	XIA Jiezhen
	CAO Rong

Cite this article:

XU Wanlin,FENG Tengrui,WU Qi, et al. Research Progress of Two-dimensional Carbon-based Material in Lithium-Sulfur Battery[J]. Materials Reports, 2025, 39(7): 23100229-10.

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https://www.mater-rep.com/EN/10.11896/cldb.23100229 OR https://www.mater-rep.com/EN/Y2025/V39/I7/23100229

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