锌电池中钴基正极材料的应用现状与挑战

doi:10.11896/cldb.23040024

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Abstract Benefiting from abundant mineral resources, ultra-high theoretical capacity and excellent safety, aqueous zinc batteries have become a strong contender for next-generation energy storage devices. As an ideal cathode material candidate for zinc batteries, cobalt-based electrode materials have received increasing attention in recent years due to their high output voltage, high theoretical capacity and excellent redox ability (Co²⁺↔Co³⁺↔Co⁴⁺). Although cobalt-based catalysts applied to zinc-air batteries have been reviewed by researchers, they mainly focus on a single catalytic direction, and a systematic summary of the multifunctional properties of cobalt-based electrode materials is lacking. This review introduces the application of multifunctional properties of cobalt-based cathode materials in zinc batteries, combining both their redox and oxygen catalysis capabilities, expanding from zinc-cobalt batteries to zinc-cobalt hybrid systems. Then, the charging and discharging mechanisms in the two battery systems are introduced, following by the current optimization strategies of cobalt-based materials in zinc-cobalt batteries and the design of electrode/electrolyte three-phase interface in zinc-cobalt hybrid batteries. Finally, this paper introduces the shortcomings of the current research and provides an outlook on future research.

Key words： cobalt-based materials zinc-cobalt battery hybrid zinc-cobalt battery

Published: 25 March 2024 Online: 2024-04-07

CLC number:

TQ152

Fund:Anhui Provincial Natural Science Foundation (2008085ME155), National Innovative Talents Program (GG2090007001), Chinese Academy of Sciences (CAS) Program (KJ2090130001), and USTC Startup Program (KY2090000044).

Corresponding Authors: ^*pengtan@ustc.edu.cn

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	SHANG Wenxu
	YU Wentao
	HE Yi
	MA Yanyi
	TAN Peng

Cite this article:

SHANG Wenxu,YU Wentao,HE Yi, et al. Current Status and Challenges in the Application of Cobalt-based Cathode Materials in Zinc Batteries[J]. Materials Reports, 2024, 38(6): 23040024-10.

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https://www.mater-rep.com/EN/10.11896/cldb.23040024 OR https://www.mater-rep.com/EN/Y2024/V38/I6/23040024

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