涉水环境材料损伤自修复策略研究进展

doi:10.11896/cldb.24010101

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Abstract Self-healing technology has emerged as a promising strategy for material damage management, and related research has been underway for nearly two decades. However most of the current self-healing strategies are primarily designed for atmospheric environments, with limited consideration for the significant influence of abundant polar water molecules in aquatic environments. Consequently, when encountering application scenarios involving water exposure, the repair effectiveness of these strategies falls short of expectations. Aquatic environments are typical and widespread special service conditions for materials used in marine engineering, hydraulic engineering, and bioelectronic devices. In recent years, researchers have gradually shifted their attention towards this issue and conducted a series of studies. This paper provides a comprehensive review of the recent research progress in self-healing strategies for material damage in aquatic environments. The focus is placed on two approaches: ‘water molecule shielding-based' (utilizing hydrophobic interactions, dipole-dipole interactions, ion-dipole interactions, and van der Waals forces) and ‘water molecule exploitation-based' (employing catechol chemistry, imine bonds, and boronic ester bonds), and an overview of their repair mechanisms is summarized. The paper also concerns an innovative discovery based on water molecule-induced accelerated self-healing and adumbrates its mechanism, and finally ends with an evaluation and outlook of research on self-healing strategies in aquatic environments.

Key words： aquatic environments material damage intrinsic self-healing water molecule shielding water molecule exploitation

Published: 25 April 2025 Online: 2025-04-18

CLC number:

TB381

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	Articles by authors
	LI Weihua
	YANG Jie
	SHEN Ting
	CHEN Chong
	WANG Zhihao

Cite this article:

LI Weihua,YANG Jie,SHEN Ting, et al. Research Progress of Self-healing Strategies for Material Damage in Water-exposed Environments[J]. Materials Reports, 2025, 39(8): 24010101-16.

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https://www.mater-rep.com/EN/10.11896/cldb.24010101 OR https://www.mater-rep.com/EN/Y2025/V39/I8/24010101

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