| INORGANIC MATERIALS AND CERAMIC MATRIX COMPOSITES |
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| Application of Layered Double Hydroxides and Their Derivatives in Lithium-Sulfur Batteries |
| GE Shiwei, ZHAO Qian*, LIU Yu, LIU Yaoyang, WEI Chu
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| State Key Laboratory of Bio-based Material and Green Papermaking, Key Laboratory of Pulp and Paper Science & Technology of Ministry of Education, Qilu University of Technology (Shandong Academy of Sciences), Jinan 250353, China |
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Abstract Lithium-sulfur (Li-S) batteries are promising next-generation energy storage systems due to their high theoretical energy density and low material cost. However, the application of Li-S batteries is hindered by the poor electrical conductivity of sulfur, the shuttle effect of polysulfide during charge-discharge process, the volume expansion and the lithium dendrites, which result in low capacity, severe capacity decay and inferior Coulombic efficiency of the batteries. Layered double hydroxides (LDHs) are two-dimensional materials with adjustable intercalation structure, controllable surface chemistry and unique topological conversion properties, which have received widespread attention in energy storage systems. In Li-S batteries, the LDHs have good confinement properties for polysulfides, which can efficiently adsorb and catalyze the polysulfides, accelerate the kinetics of the redox reaction when used as sulfur host, thus enhance the electrochemical performance of Li-S batteries. Moreover, the two-dimensional LDHs can also be used as an interlayer between cathode and separator to physically inhibit the shuttle effect of Li-S batteries. Furthermore, when used in lithium anode, the LDHs can promote the uniform nucleation and deposition of lithium metal. So, in this paper, we summarize the advantage of LDHs and their derivatives in the cathode, interlayer and anode of Li-S batteries, and point out the development direction of LDHs materials in Li-S batteries.
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Published: 25 October 2024
Online: 2024-11-05
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| Fund:National Natural Science Foundation of China (52102269), Natural Science Foundation of Shandong (ZR2020QE06), and Qilu University of Technology (Shandong Academy of Sciences) Science, Education and Industry Integration Pilot Project in Basic Research Category(2023PY008). |
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2024, Vol. 38 
