含过氧键化合物在土壤及地下水PAHs污染修复中的应用进展

doi:10.11896/cldb.22080204

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Abstract The remediation and treatment of soil and groundwater contaminated by polycyclic aromatic hydrocarbons (PAHs) is an urgent task that remains to be accomplished. The advanced oxidation technology based on peroxobond compounds has attracted constant attention because of its high efficiency in degrading PAHs in soil and groundwater. This study reviews the research on the application of hydrogen peroxide, persulfate and peracetic acid in remediating PAHs-contaminated soil and groundwater. We discuss the activation and degradation mechanisms from the perspective of free radicals generated by peroxybond breakage, explore the application prospect of peracetic acid in remediating PAHs-polluted soil and groundwater, and analyze the main external factors affecting the remediation efficiency. It is found that the types of free radicals produced vary based on different activation methods, so does their effect on PAHs pollution remediation. Moreover, the remediation effect is affected greatly by the complex environments of soil and groundwater. Therefore, in future research, new activation materials should be developed to improve the remediation effect and reduce secondary pollution. In addition, appropriate activation methods should be chosen based on the specific soil and groundwater environments, and surfactants should be used to expand the remediation range of oxidants. For that, more in-depth studies should be carried out on the remediation of PAHs pollution by peracetic acid. The remediation of PAHs-contaminated soil and groundwater by peroxybond compounds is a fruitful ground for continuing studies and a technology with broad and bright application prospect. This review provides a theoretical basis for such studies.

Key words： advanced oxidation technologies (AOPs) peroxy bond polycyclic aromatic hydrocarbons (PAHs) soil and groundwater

Published: 25 March 2024 Online: 2024-04-07

CLC number:

X53

Fund:National Key R & D Program of China (2019YFE0114900), the National Natural Science Foundation of China (42077175), and Shanghai ‘Science and Technology Innovation Action Plan' Project (19230742400, 19ZR1459300).

Corresponding Authors: ^*daichaomeng@tongji.edu.cn

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	HAN Yueming
	DAI Chaomeng
	DUAN Yanping
	LIU Shuguang
	ZHANG Yalei

Cite this article:

HAN Yueming,DAI Chaomeng,DUAN Yanping, et al. Application Progress of Peroxybond Compounds in Remediation of PAHs Pollution in Soil and Groundwater[J]. Materials Reports, 2024, 38(6): 22080204-7.

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https://www.mater-rep.com/EN/10.11896/cldb.22080204 OR https://www.mater-rep.com/EN/Y2024/V38/I6/22080204

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