| ELECTROCHEMICAL ENERGY MATERIALS AND DEVICES |
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| Mechanism of Interfacial Effects in Sodium-ion Storage Devices |
| WEI Yifan1,2, XIA Huicong1,2,*, ZHANG Jianan1,2,*
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1 College of Materials Science and Engineering, Zhengzhou University, Zhengzhou 450001, China
2 Key Laboratory of Advanced Energy Catalytic and Functional Material Preparation of Zhengzhou City, Zhengzhou 450001, China |
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Abstract Rechargeable sodium-ion batteries (SIBs) are the next generation of secondary batteries. During charging and discharging, the behavior of sodium ion (Na+) storage at the electrode interface and electrode-electrolyte interface determines the performance of SIBs, which plays an important role in the high energy density and long cycle stability required by the large-scale energy storage battery system. Although electrode materials have been extensively studied, there is very little work on the construction of stable and efficient SIBs interfaces compared to the large number of electrode materials studied. Although there are a few researches and explorations on the mechanism of interfacial effect, the researches on the regulation strategies of interfacial effect are still in the initial stage, and the results obtained are not in-depth enough to draw systematic conclusions. Here in, the mechanism of interfacial effect in Na+ storage process is reviewed. The interface is divided into heterogeneous interface of electrode material, solid electrolyte interphase and cathode electrolyte interphase. The mechanism of interfacial effect in intercalation reaction, transformation reaction and alloy reaction and its influence on the overall battery performance were summarized. This provides guidance for the optimization of electrode structure and electrode-electrolyte interface structure, which is very important for the performance optimization of SIBs. In addition, it analyzes the challenges in SIB interfacial effects research and suggests several promising methods and opportunities for advancing the understanding of interfacial effects mechanisms.
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Published: 25 April 2024
Online: 2024-04-28
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| Fund:Key Projects of the National Natural Science Foundation of China (U22A20107), the Science and Technology R & D Program Joint Fund Project of Henan Provincial (222301420001), the Distinguished Young Scholars Innovation Team of Zhengzhou University (32320275), Key Research Projects of University in Henan Province (24A150041), National Funded Postdoctoral Researcher Program (GZC20232382), and Henan Pro-vince Science and Technology Research Projects (242102240106). |
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2024, Vol. 38 
