INORGANIC MATERIALS AND CERAMIC MATRIX COMPOSITES |
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Research Progress on Defect Structure Evolution and the Corresponding Physical Mechanisms of Molybdenum Disulfide Under Electron Beam Irradiation |
JI Xuemei1, HAO Chi1, ZHU Xiumei1, SU Jiangbin1,2,3,*, HE Zuming1, TANG Bin1, ZHU Xianfang2,*
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1 Experimental Center of Electronic Science and Technology, School of Microelectronics and Control Engineering, Changzhou University, Changzhou 213159, Jiangsu, China 2 China-Australia Joint Laboratory of Functional Nanomaterials, School of Physical Science and Technology, Xiamen University, Xiamen 361005, Fujian, China 3 Key Laboratory of MEMS Education Department, School of Electronic Science and Engineering, Southeast University, Nanjing 210096,China |
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Abstract The rich polyatomic structures of molybdenum disulfide (MoS2) bestow upon it with excellent electrical, optical, and catalytic properties, arousing great interest. The defect structures in MoS2 often have a significant impact on its performance, which is generally considered to be negative. Therefore, previous studies aimed at avoiding the occurrence of defect structures. However, some recent studies have shown that MoS2 defects also have positive significance in their applications. To better leverage the defect structures of MoS2 and harness their positive impact, it is first necessary to understand these defect structures, their evolution modes and related physical mechanisms, and use them to guide the controllable nanoprocessing and practical applications. In this review, the authors summarize the different types of defect structures in MoS2 and the structural evolution behavior of MoS2 under electron beam irradiation, and then explore the mechanisms of the interaction between electron beam and MoS2 defect structures. By analyzing the limitations of traditional physical mechanisms, the authors propose two new concepts—nanocurvature effect and non-thermal activation effect to delve into the underlying physical mechanisms of these experimental phenomena. This exploration is conducted from the perspectives of nano-space limitation and ultrafast time limitation. Finally, the authors present their perspectives and prospects on defect structure modulation and controllable nanoprocessing of MoS2.
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Published: 10 February 2024
Online: 2024-02-19
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Fund:Basic Research Program of Jiangsu (Natural Science Foundation) (BK20191453) and the Graduate Research Innovation Program of Jiangsu (KYCX21_2825, KYCX21_2819). |
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