光热催化二氧化碳还原合成高附加值化学品的研究进展

doi:10.11896/cldb.22050159

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Abstract Ever-increasing fossil-fuel combustion has led to a dramatic increase in carbon dioxide (CO₂) concentrations around the globe. The concept of converting CO₂ into high-value-added chemicals such as CO, CH₄, and C₂₊ becomes great significance and urgency toward achieving carbon neutrality and carbon peaking. Photothermal catalysis as an emerging technology has gained immense attention because it combined the merits of thermal catalysis and photocatalysis. Despite these advantages, solar-to-thermal conversion efficiency and intrinsic reaction mechanism remain the technological challenges of our time. Selective suitable materials and tailored structures are favored to improve the optical properties and reduce heat losses. Accordingly, we have summarized the research and development of photothermal materials, with emphasis on the me-chanism of CO₂ conversion. Additionally, the improving strategies of photothermal catalysts including heterojunction construction, metal loading, structure regulation, and defect engineering, etc. are reviewed. It is believed that this review will provide a strategy and guidance for the construction of highly efficient photothermal materials, as well as the application in energy and environment fields.

Key words： photothermal synergistic catalysis photothermal catalytic material carbon dioxide conversion high value-added chemical

Published: 25 November 2023 Online: 2023-11-21

CLC number:

TB34

Fund:Natural Science Foundation of Jiangsu Province (BK20210867), Natural Science Research Project of Higher Education Institutions in Jiangsu Province (21KJB150038, 20KJB150042), the Doctor Project of Mass Entrepreneurship and Innovation in Jiangsu Province (202030774), and National Natural Science Foundation of China (22008163, U1604121).

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	Articles by authors
	LI Songqi
	QU Jiafu
	HU Jundie
	YANG Xiaogang
	LI Changming

Cite this article:

LI Songqi,QU Jiafu,HU Jundie, et al. Research Progress of Photothermal Catalytic CO₂ to High Value-added Chemicals[J]. Materials Reports, 2023, 37(22): 22050159-8.

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http://www.mater-rep.com/EN/10.11896/cldb.22050159 OR http://www.mater-rep.com/EN/Y2023/V37/I22/22050159

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