| POLYMERS AND POLYMER MATRIX COMPOSITES |
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| Research Progress on the Application of ZIF-derived Materials in Oxygen Reduction, Oxygen Evolution and Hydrogen Evolution Reactions |
| ZHAO Shuaikai1, LI Yaru1,2, REN Yongpeng1,2,3,*, WANG Changji1,2,3, PAN Kunming1,2,3,*, WANG Limeng1, LYU Beibei1, XIA Liangbin1, CHEN Xuemin1
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1 School of Materials Science and Engineering, Henan University of Science and Technology, Luoyang 471000, Henan, China
2 Henan Key Laboratory of High-temperature Structural and Functional Materials, National Joint Engineering Research Center for Abrasion Control and Molding of Metal Materials, Henan University of Science and Technology, Luoyang 471000, Henan, China
3 Longmen Laboratory, Luoyang 471000, Henan, China |
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Abstract Oxygen reduction reaction (ORR), oxygen evolution reaction (OER) and hydrogen evolution reaction (HER) are three vital electrocatalytic semi-reactions commonly constrained by reaction kinetics. Efficient and stable electrocatalysts can lower the reaction activation energy, enhancing the performance of new energy devices such as fuel cells, metal-air batteries and electrolytic cells. Zeolite imidazole framework (ZIF) structures possess porous structure and high specific surface area, with their derivatives have dispersed and stable active sites, which can improve catalytic performance while reducing metal consumption. This paper presents the structure-activity relationship between typical ZIF-derived material's structure, active center and properties based on their research status in the fields of ORR, OER, and HER. Firstly, the electrocatalytic mechanism and typical preparation methods of ZIF-derived materials were summarized, followed by a discussion on the effects of structure regulation and active center regulation on the catalytic performance of ZIF-derived materials. Finally, the future development and optimization design of the material for electrocatalysis were prospected.
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Published:
Online: 2023-09-06
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| Fund:National Natural Science Foundation of China (51901069), the Program for Science & Technology Innovation Talents in the University of Henan Province (22HASTIT1006), the Program for Central Plains Talents (ZYYCYU202012172), and the Ministry of Education, Singapore ( RG70/20). |
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2023, Vol. 37 
