纳米有机杂化材料(NOHMs)用于CO<sub>2</sub>捕集的研究进展

doi:10.11896/cldb.21120114

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Abstract In recent years, nano organic hybrid materials (NOHMs) have attracted widespread attention. Different from the traditional amine based solvents that capture CO₂, NOHMs can maintain liquid like properties without any solvent, with negligible vapor pressure and high thermal stability. Therefore, it is a potential substitute for traditional amine absorption because the loss caused by solvent volatilization and environmental protection problems can be reduced, and the corrosion of equipment can be avoided. At the same time, NOHMs not only are used as absorbents to absorb CO₂ directly,andbut also play a more significant role in CO₂ capture as an additive. For example, as a kind of dopant in membrane separation methods, it will play a significant role in enhancing mass transfer in CO₂ capture. This paper outlines the research progress of NOHMs in the field of carbon capture, and describes the effects of their core, corona and canopy on the CO₂ adsorption performance for two types of NOHMs connected by covalent and ionic bonds, respectively. The effects of core size, porosity, content and canopy density, chain length and structure on the capture of CO₂ by NOHMs have been discussed, and the role of enthalpy effect and entropy effect on carbon capture performance has also been summarized. The paper is expected to provide new insights and ideas in broadending applications of NOHMs in the field of CO₂ capture.

Key words： nano organic hybrid materials (NOHMs) CO₂ capture core-shell structure enthalpy effect entropy effect

Published: 25 August 2023 Online: 2023-08-14

CLC number:

TQ028.8

Fund:Natural Science Foundation of Liaoning Province, China (20170540685,2014020117), Liaoning Baiqianwan Talents Program and Key Research Projects of Liaoning Provincial Department of Education(LZGD2019004).

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	QIU Hanyu
	LIU Hongjing
	YAO Hui
	LIU Xueli
	GAO Jie

Cite this article:

QIU Hanyu,LIU Hongjing,YAO Hui, et al. Research Progress of Nano Organic Hybrid Materials (NOHMs) for CO₂ Capture[J]. Materials Reports, 2023, 37(16): 21120114-11.

URL:

http://www.mater-rep.com/EN/10.11896/cldb.21120114 OR http://www.mater-rep.com/EN/Y2023/V37/I16/21120114

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