NASICON结构Na3Zr2Si2PO12固体电解质研究进展

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Abstract The progress of social science and technology has promoted the rapid development of battery energy storage technology. The requirements of various electronic components in life for energy storage batteries are also increasing. It is the most urgent task to develop energy storage materials with high energy density and high safety. However, the current secondary batteries mostly use organic electrolyte, which is prone to leakage and erosion of electrodes, and may explode at high temperature. Using solid electrolyte to develop all-solid-state batteries is not only beneficial to the miniaturization and diversification of products, but also can avoid the problems of liquid electrolyte and greatly reduce the security risks. Na₃Zr₂Si₂PO₁₂ ( NZSP ) of NASICON (Na⁺ super ionic conductor)-structure is one of the most promising solid electrolyte materials at pre-sent, which has the advantages of isotropic, non-reaction with Na, high conductivity and high decomposition voltage.In this paper, the research progress of Na₃Zr₂Si₂PO₁₂ solid electrolyte with NASICON-structure in recent years is reviewed from the four aspects of NZSP crystal structure and ion diffusion mechanism, synthesis method, ion doping modification and NZSP solid electrolyte/electrode interface modification. Finally, difficulties and challenges encountered in the development of Na₃Zr₂Si₂PO₁₂ solid electrolyte are summarized, with the solution direction provided.

Key words： electrolyte material ion doping Na₃Zr₂Si₂PO₁₂ NASICON (Na⁺ super ionic conductor)-structure

Published: 05 June 2022 Online: 2022-06-08

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TM911

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	Articles by authors
	ZHAO Yuhui
	ZHANG Yarong
	WU Yongmin
	ZHU Lei
	GUO Jun
	TANG Weiping

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ZHAO Yuhui,ZHANG Yarong,WU Yongmin, et al. Research Progress of Na₃Zr₂Si₂PO₁₂ Solid Electrolyte with NASICON-structure[J]. Materials Reports, 2022, 36(Z1): 21050235-9.

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http://www.mater-rep.com/EN/ OR http://www.mater-rep.com/EN/Y2022/V36/IZ1/21050235

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