低膨胀β-锂霞石基复合材料的研究现状与进展

doi:10.11896/cldb.18100095

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Abstract Thermal expansion coefficient is one of the important parameters of materials. In nature, most materials exhibit high thermal expansion coefficient which would lead to the phenomenon of thermal-expansion and cold-contraction. Therefore, these materials usually have poor thermal shock resistance and cannot be used in the environment with great temperature changes. The signal distortion usually occurs because of the destruction of aerospace components and the deformation of electronic device resulted from the uneven temperature distribution. It is exciting that there are a few materials with negative thermal expansion coefficient, and their volume decreases with the increase of temperature. Based on the additivity of the expansion coefficient, the compounds with low coefficient of thermal expansion can be obtained by introducing the material with low or negative coefficient of thermal expansion into the high ones, which can remarkably improve their thermal shock resistance.
　　Negative thermal expansion materials include isotropic negative thermal expansion materials and anisotropic negative thermal expansion mate-rials. Isotropic negative thermal expansion materials are mainly ZrV_2-xP_xO₇ and ZrW₂O₈ series. Anisotropic negative thermal expansion materials mainly include β-eucryptite, perovskite series, A₂M₃O₁₂series, M(CN)₂ (M=Zn, Cd) series, oxides, zeolite series and metal organic frameworks (MOFs), etc.
　　The β-eucryptite is usually used to adjust the thermal expansion coefficient of composite materials owing to its negative thermal expansion coefficient (α=-6.1×10^-6 K^-1), low density (2.67 g/cm³), good thermal shock resistance, dielectric properties and infrared radiation. Composite materials with negative thermal expansion or near zero thermal expansion can be fabricated by compounding with other materials, which can greatly improve the thermal shock resistance and dimensional stability of the materials, and thus prolong the life of the materials. Therefore, β-eucryptite has been used to manufacture low expansion ceramics, glass-ceramics, metal matrix composites applied as fillers for electrical equipment, electronic components, device sealants, aircraft high precision components, humidity sensor sensitive materials and lithium ion battery so-lid electrolytes. At the same time, due to the anisotropic thermal expansion property of β-eucryptite, the composites will have more residual stress and lower mechanical strength. In order to solve this problem, fibers or whiskers with high mechanical strength can be introduced to form three-phase composites with low expansion and high mechanical strength, which is beneficial to expand the application of materials in inertial missiles, optic fiber gyro and other aerospace applications. In this paper, the research status and progress of the low expansion two-phase or three-phase composites of metals, glass and ceramics are reviewed. The preparation method, thermal properties and application fields of these low expansion coefficient composites are summarized. The future development trends and application prospects of the composites are also discussed.

Key words： β-eucryptite negative thermal expansion composites

Published: 16 January 2020

CLC number:	TQ175.4
	TD985
	TB35

About author:: Yaohui Xuereceived his M.S. degree of material scie-nce from Tsinghua University in 2005 and received his Ph.D. degree in microelectronics and solids state electronics from Xi’an Jiaotong University in 2012.He is currently a senior engineer in Xi’an Modern Control Technology Research Institute. His research interests are optical fiber communication technology and optical fiber sensing technology;Xiaoxia Cuireceived her Ph.D. degree in optics from the Xi’an Institute of Optics and Precision Mechanics, Chinese Academy of Sciences, in 2010. She is currently a full associate professor in State Key Laboratory of Transient Optics and Photonics in Xi’an Institute of Optics and Precision Mechanics. Her research interests are functional nano-materials and nano-composites.

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Cite this article:

XUE Yaohui,JIANG Junbiao,ZHANG Hui, et al. Research and Progress of Low-expansion β-eucryptite Composites[J]. Materials Reports, 2020, 34(5): 5068-5077.

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http://www.mater-rep.com/EN/10.11896/cldb.18100095 OR http://www.mater-rep.com/EN/Y2020/V34/I5/5068

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