柔性储能器件的电极设计研究进展

doi:10.11896/cldb.19110021

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Abstract In light of the rapid development of electronic technologies, portable electronic devices are promoted to evolve with fascinating flexibility, mi-niaturization and intellectualization. Flexible electronics with the features of bent, folded, twisted, stretched and coordinated deformations are now the booming fields of research. As a crucial component of flexible electronic devices, the design of reliable energy storage systems has become the key challenges towards the applications of flexible electronics. Traditional energy storage devices are rigid, which is easy to break under applied deformations. Accordingly, the separation of electrode materials and current collector seriously deteriorates the electrochemical perfor-mances and even causes a short circuit, resulting in safety issues. To this end, flexible energy storage devices, such as flexible Li-ion batteries, flexible Li-S batteries and flexible lithium metal batteries, have gained paramount interests in academia and industry.
In recent years, great progress has been made in flexible energy storage devices based on intrinsic flexible materials assembly andrigid mate-rials flexible designs. Metal fibers (e.g., Al and Cu), polymer fibers (e.g., polypyrrole and polyaniline), and carbon-based materials (e.g., carbon nanofibers, carbon nanotubes and graphene) have so far been widely applied in flexible energy storage devices because of their intrinsic fle-xibility. While the other materials with the characteristics of brittleness, for example, lithium cobaltate and lithium titanate, can achieve a certain degree of flexibility after reasonable structural design. In addition, the practical application of flexible energy storage systems must meet the crite-rions in terms of high capacity, high efficiency, light weight, high safety and so on.
This review dedicates to discuss the relationships between the microstructure of nanomaterials and the performance of devices. The preparation methods, mechanical properties and electrochemical performances of current flexible systems are briefly overviewed. Moreover, instructive perspectives are provided so that to enlighten more insightful contributions to flexible electronics.

Key words： flexible electronics electrochemical energy storage electrode materials intrinsic flexibility extrinsic flexibility

Published: 15 January 2020

CLC number:

TB34

Fund:This work was supported by the National Natural Science Foundation of China (51902261), the Natural Science Basic Research Program of Shaanxi (2019JQ-025), Fundamental Research Funds for the Central Universities (31020180QD094, 31020180QD116).

About author:: Yifan Li received his B.E. degree in Material Forming and Control Engineering from Taiyuan University of Science and Technology in 2019. He is currently a master student in the Institute of Flexible Electronics at Northwestern Polytechnical University under the supervision of Prof. Wei Ai. His research is focused on new energy devices and flexible energy storage.
Yuhang Liu received his M.S. degree in School of Physical Science and Technology, Lanzhou University. He is currently pursuing his Ph.D. degree under the supervision of Academician Prof. Wei Huang and Prof. Wei Ai in the Institute of Flexible Electronics, Northwestern Polytechnical University. His research interests involve the design and synthesis of carbon nanofibers-based electrodes for Li-ion batteries and lithium metal battery.
Wei Ai received his Ph.D. and M.S. degrees from Nanyang Technological University and Nanjing University of Posts and Telecommunications, respectively. After working as a research associate at Nanyang Technological University, he joined in the Institute of Flexible Electronics at Northwestern Polytechnical University. His research interests focus on electrochemical materials and technologies, new energy devices, flexible intelligence technologies, etc.
Wei Huang received his B.S., M.S., and Ph.D. degrees in Chemistry from Peking University in 1983, 1988, and 1992, respectively. In 2001, he became a chair professor at Fudan University, where he founded the Institute of Advanced Materials (IAM). In 2006, he was appointed as the Deputy President of Nanjing University of Posts and Telecommunications. He was elected as the academician of Chinese Academy of Sciences in 2011. In 2012, he was appointed as the President of Nanjing Tech University. Now he is the deputy president and provost of the Northwestern Polytechnical University. His research interests include flexible electronics, organic optoelectronics, nanoelectronics, and bioelectronics.

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	LI Yifan
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Cite this article:

LI Yifan,LIU Yuhang,SUN Jinmeng, et al. Progress of Electrode Designs for Flexible Energy Storage Devices[J]. Materials Reports, 2020, 34(1): 1177-1186.

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http://www.mater-rep.com/EN/10.11896/cldb.19110021 OR http://www.mater-rep.com/EN/Y2020/V34/I1/1177

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