碳酸化钢渣及其在建筑材料中的应用现状

doi:10.11896/cldb.19040004

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Abstract As global warming receives more and more attention, greenhouse gas carbon dioxide (CO₂) emissions, capture and storage are also receiving increasing attention. Mineral carbonation technology refers to the acceleration reaction between alkaline minerals in nature with CO₂ to form stable carbonates by specific technology. It has became a promising CO₂ storage technology due to the stable and environmentally friendly carbonation products. However, natural minerals show low carbonation activity and low CO₂ uptake. In addition, CO₂ emitted from fossil fuel combustion requires a large amount of natural resources and high energy to form carbonates. The above-mentioned disadvantages hinder the development of mineral carbonation technology. Alkaline industrial waste such as steel slag is proposed to replace natural alkaline minerals for mineral carbonation. It provides a feasible way to reduce CO₂ emissions, and also provides a new resolution for the utilization of industrial waste.
The CO₂ uptake and carbonation rate of steel slag are affected by many factors. In recent years, domestic and foreign scholars have done a lot of work to explore carbonation mechanism of steel slag, optimize the parameters of carbonation process, increase CO₂ uptake, reduce energy consumption, and have achieved fruitful results. However, China produces a large amount of steel slag every year and the utilization is limited. If steel slag is only used for CO₂ capture, it will increase the bulk density of steel slag and further increase the difficulty of steel slag treatment, and in addition, steel slag cannot be used efficiently. Therefore, many researchers have developed a carbonation curing technology to prepare building materials to realize the utilization of steel slag, in order to solve the problem of poor volume stability when steel slag is applied in building materials.
Carbonation mechanism of steel slag, carbon sequestration ability and characteristics of different alkaline minerals in steel slag, and the mea-sures to increase carbon sequestration of steel slag are reviewed in this paper. In addition, the application of carbonated steel slag in building materials and the effects of carbonation on the mechanical properties and microstructure of steel slag are introduced. The prospects, technical difficulties and challenges of applying carbonated steel slag in building materials are discussed.

Key words： carbon dioxide (CO₂) carbonation steel slag mechanical properties microstructure building materials

Published: 03 January 2020

CLC number:

TU528

Fund:This work was financially supported by National Natural Science Foundation of China (51808354), Natural Science Foundation of Liaoning Province (20180550127), China Postdoctoral Science Foundation(2018M641712) and State Key Laboratory of Silicate Materials for Architectures (Wuhan University of Technology).

About author:: Yanfeng Fang received her Ph.D. degree from Dalian University of Technology in 2017 and she is a lecturer in Shenyang Jianzhu University. Her research interests are industrial waste utilization and special cementitious materials. In recent years, she has presided 5 projects including 1 National Natural Science Foundation projects, 1 Liaoning Provincial Natural Science Foundation projects. And she has participated in 3 provincial and ministerial level projects about building materials;Jun Chang is a full professor and doctoral supervisor in Dalian University of Technology. His research interests are special cement and concrete materials, comprehensive utilization of waste residue and cement-based functional materials. He hosted and participated in more than 10 research projects including National 863 project, National 973 project, National Natural Science Foundation and provincial and ministerial level projects. He has won 7 national and provincial-level science and technology awards including the second prize of national technology invention, the second prize of scientific and technological progress of the national building materials industry, the first prize of Shandong Science and Technology Progress Award, and the first prize of Shandong Province Technology Invention. In 2005, he was awarded “Outstanding Young Intellectuals of Shandong Province”. In 2010, he won the Shandong Youth Science and Technology Award. In 2010, he was selected as the New Century Excellent Talent Support Program of the Ministry of Education.

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Cite this article:

FANG Yanfeng,WANG Dan,WANG Qing, et al. A Review on Carbonation of Steel Slag and Its Application in Building Materials[J]. Materials Reports, 2020, 34(3): 3126-3132.

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http://www.mater-rep.com/EN/10.11896/cldb.19040004 OR http://www.mater-rep.com/EN/Y2020/V34/I3/3126

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