基于生物精细构型的光催化材料和光热转换材料的研究进展

doi:10.11896/cldb.18100186

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Abstract  The global energy crisis and environmental pollution have long come to the foreground of our attention. As a kind of renewable energy, clean, low-cost and efficient solar energy conversion and utilization are of great significance. The solar energy can be converted into hydrogen energy which can be stored and transported through the photocatalysis, and the sea water can be desalinated by the solar energy through the photothermal effect. Both of them can help to alleviate the problems of energy shortage, environmental pollution and shortage of fresh water resources and the like.
    How to improve the energy conversion efficiency oflight energy conversion materials is a key issue in the field of solar energy conversion. The properties of materials depend on a number of factors, among which configuration is one of the most important factors. Therefore, excellent material configuration design has become a research hotspot in many fields such as materials, chemistry, biology, etc., to attain the requirements for applications of photocatalysis, photothermal therapy, energy conversion and storage. However, at present, the main methodology of artificial preparation are “bottom-up” chemical self-assembly and “top-down” physical processing. Both of them are unlikely to balance both cost and efficiency and obtain hoped-for configurations. In view of this, some scholars put forward the concept of “Morphology genetic materials”, which refers to the fine configuration of natural organisms (including microorganisms, animals and plants).And, they have advocated utilizing the structure of natural organisms as template to prepare materials with special structures and functions, which had provided distinctive insights and inspiration for scientific research in many fields nowadays.
    In recent years, solar energy conversion materials based on biological fine configuration have developed rapidly, and a large number of outstanding achievements have emerged in the field of photoelectrocatalysis and photothermal conversion.Inspired by photosynthesis in nature, solar energy can be converted to chemical energy by photocatalysis reactions. Materials with three-dimensional hierarchical structure exhibits good anisotropy, large reaction contact area and sufficient micro-nano pores, which can effectively enhance the electrical, optical and catalytic properties of semiconductor. Micro-nano porous structure materials with leaves, butterflies and others organisms as templates could improve the absorption of incident light of the catalyst, and also provide more reaction sites for water splitting. The hydrogen production performance is several times hig-her than that of materials with common configuration. At the same time, in the photo-thermal water evaporation system, the composite materials consist of metal nanoparticles and butterfly wings, lotus or other templates show excellent photothermal evaporation rate and conversion efficiency due to the rapid water absorption capacity, efficient light absorption, light enhancement ability and good thermal insulation ability of biological templates. In this paper, construction and application of solar energy efficient conversion materials based on biological fine configuration such as lea-ves, butterflies, diatoms, etc. are summarized, including their application in photocatalytic water decomposition and light-driven water evaporation. This paper could provide valuable information for the study in design and preparation of light energy conversion materials with graded micro-nano configurations.

Key words： solar energy conversion biological fine configuration photocatalysis photothermal conversion

Published: 12 September 2019

CLC number:

TB383.1

Fund:This work was financially supported by the National Natural Science Foundation of China (51772187, 51271116, 51572169, 51672175), Key Program for International S&T Cooperation Program of China (2017YFE0113000), Shanghai Science and Technology Committee (18JC1410500, 17ZR1441400, 17520710600, 16520710900)

About author:: Cheng Sun received his B.S. degree in materials scie-nce and engineering from Shanghai Jiao Tong University in 2016. He is currently pursuing his master's degree at the State Key Lab of Metal Metrix Composites, Shanghai Jiao Tong University under the supervision of Prof. Jiajun Gu. His research has focused on application of morph-genetic materials in the fields of photocatalysis and photothermal conversion.
Jiajun Gu received his B. E and Ph. D degrees from Shanghai Jiao Tong University (SJTU) in 1996 and 2005, respectively. During 2001—2003, he spent 18 months studying at Kyoto University, Japan (Monbusho Scholarship). He started his research career with the team of Morphogenetic Materials headed by Prof. D. Zhang at Shanghai Jiao Tong University in 2005, and is presently an associate professor at SJTU. In the past five years, Dr. Jiajun Gu has published more than 20 peer-reviewed papers in Angew. Chem., Adv. Funct.Mater., J. Mater. Chem., Langmuir, Appl. Phys. Lett., and Phys. Rev. B, et al. Recently, his work “Versatile fabrication of intact three-dimensional metallic butterfly wing scales with hierarchical sub-micrometer structures” (Angew. Chem. Int. Ed. 2011, 50, 8307) was highlighted by Nature as “Materials: Butterfly wings turned to metal” (Nature, 2011, 476, 9). His research interests mainly focused on the bio-inspired functional materials and solutions, either in designing and preparing novel structures, or in exploring the chemical and physical mechanisms of the synthesized products.
Di Zhang, Chang Jiang Scholars Program Professor, Executive Director of Chinese Compostie Materials So-ciety, Professional Committee of Metal Matrix and Ceramic Matrix Composites. Professor Zhang is the leader of many domestic research projects such as, National Natural Science foundation of China, 973 plan, 863 plan, and inter-government collaboration projects. At the same time his group cooperates well with many world-famous universities and companies, such as Rio Tinto Alcan (Canada), Bayer (German), Morgan Crucible (the United Kingdom), The Dow Chemical Company (the United States of America) and Toyota Company (Japan). Professor Zhang's research fields are process of advanced metal matrix composites, basic and applied research of Morph Genetic materials.

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Cite this article:

SUN Cheng,GU Jiajun,ZHANG Xiaohui, et al. Research Progress of Photocatalytic Materials and Photothermal ConversionMaterials Based on Biological Fine Configuration[J]. Materials Reports, 2019, 33(21): 3662-3668.

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http://www.mater-rep.com/EN/10.11896/cldb.18100186 OR http://www.mater-rep.com/EN/Y2019/V33/I21/3662

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