低维氧化锌晶面调控及催化抗菌活性研究进展

doi:10.11896/cldb.201901006

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Abstract As a kind of typical wide-band-gap semiconductor material, low dimensional zinc oxide (ZnO) has attracted increasing attention in long-term antibacterial, catalytic degradation and energy conversion, owing to its unique morphological adjustability, excellent catalytic activity and good biocompatibility. Sufficient research has indicated that, by changing the reaction conditions, the morphology and structure of ZnO can be easily tuned, which will further exert remarkable influence on properties and performance of ZnO. Therefore, the regulation of morphology and structure has been regarded as a crucial issue for the application of ZnO.
The morphological diversification of ZnO originates from the anisotropic growth of its crystal. Many factors (like solvent, nucleating agent and additive agent etc.) may impact on this process and facilitate the growth of crystal along different crystal orientation. Therefore, the reaction condition determines both morphology and exposed crystal facet of ZnO. The atomic alignment, atomic density and surface dangling bonds vary consi-derably among different types of crystal facets. Hence, the performance of ZnO can be regulated by carefully control the morphology, structure, crystal orientation and exposed crystal surface.
The continuous advancement of technology and simulation, the methodologies for facets regulation can be classified into crystal facets adsorption, seeding induction, solvent adjustment and crystal facets etching. The former three methods are bottom-up synthesis techniques, which achieve the control of crystal morphology and facets by either introducing adsorbents and/or seeds synthesis process, or carefully choosing appropriate solvent. On the other hand, crystal facets etching is a top-down process. The crystal facets of ZnO can be selectively etched because of the differences in reactive activity, which facilitates to obtain the required facets. These methods enable researchers to precisely regulate the crystal morphology and facet of the synthesized ZnO, and in consequence, to further study the relationship and mechanism between exposed crystal facets and catalytic antibacterial activity.
In this review, we summarize the recent progress and the common methods, along with their action mechanisms, with respect to facets regulation of ZnO. The potential effects of crystal facets regulation on the catalytic antibacterial activity of ZnO with or without light irradiation are also explored. The paper ends with a discussion on the growing trends and emerging challenges in this field.

Key words： zinc oxide exposed crystal facets facets regulation catalytic antibacterial activity crystal facets adsorption seeding induction crystal facets etching

Published: 24 January 2019

CLC number:	TB34
	O793

Fund:This work was financially supported by the National Natural Science Foundation of China (51772251,51302230), the Science and Technology Planning Project of Sichuan Province (2016GZ0264,2017RZ0032), and the support by the Fundamental Research Funds for the Central Universities (2682016CX068).

About author:: Dan Li got her Master Degree in the School of Materials Science and Engineering, Southwest Jiaotong University, Sichuan, China. Her research focuses on catalytic antibacterial materials.Zuowan Zhou is now the distinguished professor of materials science at Southwest Jiaotong University (SWJTU). He received his Ph.D. from Donghua University (Shanghai, China, 2002) in material science. Professor Zhou lead a research group on functional polymers, nanomaterials and eco-materials, in which more than 70 proposals have been permitted and acquire high opinions for the finished projects. He has published more than
200 papers and 5 books (editor, co-author for chapters or sections), and obtained about 30 items of Chinese invention patents. In recent years, Prof. Zhou presented 30 invited talks and took academic positions at international conferences and/or symposiums, and organized 10 Conferences.

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	LI Dan
	ZHANG Minhao
	LIAO Peizi
	XIE Yuan
	ZHEN Hewei
	XU Xiaoling
	ZHOU Zuowan

Cite this article:

LI Dan,ZHANG Minhao,LIAO Peizi, et al. Recent Progress in Facets Regulation and Catalytic Antibacterial Activity of Low-dimensional ZnO Crystals[J]. Materials Reports, 2019, 33(1): 56-64.

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http://www.mater-rep.com/EN/10.11896/cldb.201901006 OR http://www.mater-rep.com/EN/Y2019/V33/I1/56

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