球型Si基碳包覆锂离子电池负极材料研究进展

doi:10.11896/cldb.23020231

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Abstract Silicon-based materials, including elemental silicon and its oxide SiO_x(0≤x≤2), are expected to replace graphite as a new generation of anode material for lithium-ion batteries because of their high theoretical capacity, low working potential, environment-friendly and abundant reserves. However, the volume expansion effect of silica-based materials in the process of charge and discharge is inevitable. In addition, the low conductivity of silica-based materials also limits the development of silica-based materials. In order to solve the above problems, researchers have proposed a variety of solutions, among which the carbon coating method on the surface of silicon-based materials has a great application prospect and has been widely studied. This paper first outlines the lithium storage mechanism and failure problems of each silicon-based material, and then summarizes different spherical carbon coating structures in detail from the perspective of the most typical spherical structure design, such as core-shell structure, yolk-shell structure, porous structure, etc. The future development trend of carbon-coated anode materials based on Si and the challenges to be faced are discussed.

Key words： lithium-ion battery spherical silicon-based material carbon coating

Published: 10 November 2024 Online: 2024-11-11

CLC number:

O469

Fund:National Natural Science Foundation of China (22162008) and the Basic Research Program of Science & Technology Department of Guizhou Province ([2020]1Y055).

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	Articles by authors
	LI Donglin
	YANG Wanliang
	CAO Rui
	YANG Xue
	XU Meisong

Cite this article:

LI Donglin,YANG Wanliang,CAO Rui, et al. Research Progress of Spherical Si-based Carbon-coated Anode Materials for Lithium-ion Batteries[J]. Materials Reports, 2024, 38(21): 23020231-11.

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http://www.mater-rep.com/EN/10.11896/cldb.23020231 OR http://www.mater-rep.com/EN/Y2024/V38/I21/23020231

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