二氧化锰基催化剂催化氧化甲苯的进展

doi:10.11896/cldb.23030015

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Abstract Owing to industrial development and increasing energy consumption in China, toluene pollution has become a serious environmental concern. Among the existing toluene treatment methods, catalytic oxidation is undoubtedly the most economical and effective technical approach. The performance of the catalyst, which is the core of the catalytic reaction, is particularly essential. Although noble metal catalysts possess excellent catalytic activity, their high cost and the decrease in activity due to sintering and poisoning hinder their widespread application in industry. In recent years, manganese dioxide (MnO₂) has attracted much attention as a transition metal oxide catalyst for the catalytic oxidation of toluene owing to its high catalytic activity, thermal stability, low cost, and easy synthesis, as well as the availability of various crystal forms. However, the catalytic activity of single MnO₂ is unsatisfactory, prompting the present study on its modification and optimization. We analyzed the effects of the structural characteristics of MnO₂, such as the crystal structure, surface properties, and specific crystalline surfaces, on the catalytic efficiency of toluene. Further, we aimed to improve the performance of MnO₂ for the catalytic oxidation of toluene through modification approaches like doping and composite loading and to elucidate the catalytic oxidation mechanism of toluene on MnO₂. The direction of future research on the preparation of novel MnO₂ catalysts for toluene catalysis is outlined herein.

Key words： MnO₂ catalyzing toluene catalytic mechanism influencing factor modification and optimization

Published: 10 July 2024 Online: 2024-08-01

CLC number:	X511
	TQ-9

Fund:National Key Research and Development Program(2018YFB0604204)and Shanghai Science and Technology Tackling Project(21DZ1207203).

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	Articles by authors
	SONG Jie
	DING Honglei
	PAN Weiguo
	ZHANG Kai
	MA Junchi
	ZHANG Ziyi

Cite this article:

SONG Jie,DING Honglei,PAN Weiguo, et al. Advances in the Catalytic Oxidation of Toluene by MnO₂-based Catalysts[J]. Materials Reports, 2024, 38(13): 23030015-11.

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http://www.mater-rep.com/EN/10.11896/cldb.23030015 OR http://www.mater-rep.com/EN/Y2024/V38/I13/23030015

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