全无机CsPbBr<sub>3</sub>钙钛矿太阳电池的研究进展

doi:10.11896/cldb.20060145

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Abstract Since the first report in 2009, organic-inorganic hybrid perovskite solar cells (PSCs) have seen the improved power conversion efficiency (PCE) from 3.8% to 25.5%, which can be comparable to the commercial crystalline silicon solar cells. They have attracted tremendous attention of researchers all over the world. However, due to the weak-bonded organic components in the hybrid crystal structure, the long-term stability of devices is greatly affected. In recent years, using inorganic Cs⁺ ion to completely replace organic groups to form all-inorganic perovskites is considered to be an effective way to solve the problem of instability. Among Cs-based perovskites, CsPbBr₃ perovskite has the most excellent heat, ultraviolet light and moisture resistance, which is potentially expected to form the top cell of tandem solar cells with long-life crystalline silicon solar cells. In this paper, we systematically reviewed the research progress of CsPbBr₃ PSCs. Firstly, the history of CsPbBr₃ PSCs, and the crystal structure and basic properties of CsPbBr₃ are briefly introduced, and then the preparation methods of CsPbBr₃ thin films, element doping modification of CsPbBr₃, interface engineering of devices, and other aspects of the research progress to promote the PCE are elaborated. Finally, the current issues and the future prospect of improving the performance of CsPbBr₃ PSCs are discussed, which will provide a feasible reference to further promote the practical process of perovskite solar cells.

Key words： all-inorganic perovskite solar cells CsPbBr₃ long-term stability

Published: 25 June 2021

CLC number:

TB34

Fund:This work was financially supported by the Natural Science Foundation of Hunan Province (2020JJ4097), China Scholarship Council 2017(3059) and International Cooperation Scientific Research Project of Changsha University of Science and Technology (2018IC15).

About author:: Zhuang Liu received his B.S. degree from Changsha University of Science and Technology in 2018. He is currently pursuing his master’s degree in the School of Energy & Power Engineering, Changsha University of Science and Technology, under the supervision of associate professor Jianlin Chen. His research is currently focusing on flexible perovskite solar cells.

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	LIU Zhuang
	CHEN Jianlin
	HUANG Caiyou
	PENG Zhuoyin
	HE Jianjun
	CHEN Jian

Cite this article:

LIU Zhuang,CHEN Jianlin,HUANG Caiyou, et al. Progress of All-inorganic CsPbBr₃ Perovskite Solar Cells[J]. Materials Reports, 2021, 35(11): 11039-11056.

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http://www.mater-rep.com/EN/10.11896/cldb.20060145 OR http://www.mater-rep.com/EN/Y2021/V35/I11/11039

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