| MULTI SCALE RARE EARTH CRYSTAL MATERIALS AND THEIR APPLICATIONS |
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| Recent Advances and Perspective on Rare Earth Element Modified Lithium-based Oxide Solid Electrolytes |
| ZHANG Jiaqing1,2,3,†, ZHANG Da1,2,3,†, CHEN Kunfeng4,*, XUE Dongfeng5,*, LIANG Feng1,2,3,*
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1 Key Laboratory for Nonferrous Vacuum Metallurgy of Yunnan Province, Kunming University of Science and Technology, Kunming 650093, China
2 National Engineering Research Center of Vacuum Metallurgy, Kunming University of Science and Technology, Kunming 650093, China
3 Faculty of Metallurgical and Energy Engineering, Kunming University of Science and Technology, Kunming 650093, China
4 State Key Laboratory of Crystal Materials, Shandong University, Jinan 250100, China
5 Multiscale Crystal Materials Research Center, Shenzhen Institute of Advanced Technology, Chinese Academy of Science, Shenzhen 518055, Guangdong, China |
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Abstract All-solid-state lithium batteries have been a hot topic of research in the field of new energy because of their high energy density and high safety.The solid electrolyte, which is the key component of all-solid-state lithium battery, has significant influence on the energy density, cycle stability and safety of the battery. Among solid electrolytes, oxide solid electrolytes possess many merits of the high ionic conductivity, wide electrochemical window, and excellent mechanical property, including garnet-type, NASICON-type and perovskite-type solid electrolytes. However, the high sintering temperature, low ionic conductivity at room temperature, and unstable structure of oxide solid electrolytes cannot meet demands of the practical application. In this review, the research status and existing problems of garnet-type, NASICON-type and perovskite-type solid electrolytes in recent years are summarized. The functions of rare earth elements with large ionic radius, high valence, low electronegativity, variable coordination number and special electronic structure of 4f5d modified oxide solid electrolytes are concluded, including increasing the relative density, improving the ionic conductivity, and stabilizing the high ionic conductive crystal phase. The main scientific problems and technical bottlenecks of rare earth modified oxide solid electrolytes are analyzed. Finally, the future development direction of rare earth modified oxide solid electrolyte is prospected.
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Published: 10 February 2023
Online: 2023-02-23
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| Fund:The National Natural Science Foundation of China (12175089, 12205127, 51832007, 52220105010, M-0755), the Key Research and Development Program of Yunnan Province (202103AF140006), and the Applied Basic Research Programs of Yunnan Provincial Science and Technology Department (202001AW070004). |
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