INORGANIC MATERIALS AND CERAMIC MATRIX COMPOSITES |
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Research Progress in Synthesis and Catalytic Application of High Entropy Oxides |
YOU Zijuan1, CHEN Hanlin2,*
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1 College of Chemistry, Guangdong University of Petrochemical Technology, Maoming 525000, Guangdong, China 2 College of Environmental Science and Engineering, Guangdong University of Petrochemical Technology, Maoming 525000, Guangdong, China |
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Abstract High entropy oxides (HEOs) are composed of five or more kinds of oxides in equal or nearly equal mole and have been widely concerned by researchers at home and abroad in recent years due to its simple structure and excellent performance. The solid solution structures of HEOs mainly included rock salt, fluorite, spinel or perovskite structure oxides, which have a very broad application prospect in the field of catalysis, such as thermocatalysis, electrocatalysis and photocatalysis. Here, the synthesize methods (e.g. solid-state reaction, nebulized spray pyrolysis, flame spray pyrolysis, wet chemical and solution combustion synthesis, etc.) are introduced and their advantages and disadvantages are also compared. In addition, the main characterization methods of HEOs are described briefly. Then, the applications of HEOs in thermocatalysis, electrocatalysis and photocatalysis are summarized. More important, the reaction mechanism is analyzed to further promote the development of this emerging field. Furthermore, the theoretical calculation of HEOs are briefly introduced. Finally, the future directions and challenging perspectives for chemical catalysis over HEOs are also put forward.
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Published:
Online: 2023-12-19
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Fund:National Natural Science Foundation of China (22106023), Projects of Maoming City Science and Technology Planning(2022045), Projects of Talents Recruitment of GDUPT (2020rc015). |
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