| ENVIRONMENTAL CATALYTIC MATERIALS |
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| Photocatalytic Degradation for Benzene Series in Wide-band Gap Metal Oxide: Reaction Mechanism and Modification Strategies |
| CHEN Lyucun1,2, CUI Wen1, CHEN Peng1, LI Kanglu1, DONG Fan1,2, WANG Fali3
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1 Center of Environmental and Energy Catalysis, University of Electronic Science and Technology of China, Chengdu 610000, China
2 Yangtze Delta Region Institute (Huzhou),University of Electronic Science and Technology of China, Huzhou 313000, China
3 Ecological Environment Monitoring Station of Chongqing Wansheng Economic and Technological Development Zone, Chongqing 400800, China |
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Abstract Benzene compounds are widely present in water bodies and atmospheric environments, and their refractory and highly toxic characteristics pose a serious threat to human health and the ecological environment. Photocatalytic technology has attracted much attention in pollutant degradation and energy conversion because of mild reaction conditions, strong redox ability, and green and no secondary pollution, especially for the treatment of refractory benzene series.
The advantages of positive valence band position, strong oxidation ability, high photochemistry stability and lower cost on wide-band gap photocatalysts play important role in benzene series degradation. However, wide band gap photocatalysts have limited photo-response range, higher surface potential and difficult separation of photo-generated electron-hole pairs, which limit their application in actual treatment processes. In addition, the effects of wide variety of benzene series, complex structure, and the current in-situ characterization technology limited the understanding of the conversion and ring opening mechanism of benzene series. That restricts the design and preparation for efficient photocatalysts and photocatalytic technology for the practical application in benzene treatment.
This review focuses on the important progress about wide-band gap photocatalytic oxidation technology in the degradation of benzene series, and introduces the latest developments about the reaction mechanism of photocatalytic benzene series degradation, the performance influencing factors of wide-band gap semiconductors, and the modification strategies on wide-band gap semiconductors. Finally, the prospects in reaction mechanism research, degradation efficiency enhancement and practical application are put forward.
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Published: 30 November 2021
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| Fund:National Natural Science Foundation of China (21822601, 22006009),Sichuan Science and Technology Innovation Seedling Project Funding Project(2021077),Chongqing Science and Technology Commission Fund (cstc2019jscx-msxmX0374). |
About author:: Lyucun Chen received his Ph.D. degree in 2018 from Southwest Petroleum University. Now he is a postdoctor in the materials science and engineering at the University of Electronic Science and Technology of China, coo-perating with Prof. Fan Dong. His work focuses on the development of novel photocatalysts for environmental and energetic applications.
Fan Dong received his Ph.D. degree in 2010 from Zhejiang University. Currently, he is a full professor and doctoral supervisor at Institute of Fundamental and Frontier Sciences, University of Electronic Science and Technology of China (UESTC). His research interests include photocatalysis, environmental and energy catalysis. |
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