量子点在光电化学传感器中的研究进展

doi:10.11896/cldb.20090134

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Abstract Quantum dots are a newly developed class of photoelectric active materials. Due to unique photoelectric effect and stability, quantum dots can not only realize the conversion of light energy into electric energy, which improve the sensitivity of electrochemical detection, but also generate photocurrent at the applied voltage of about 0 V, which achieves the friendly voltage for biomolecule detection. On these grounds, quantum dots provide a new opportunity for the development of photoelectrochemical sensors.
However, the research of quantum dots in photoelectric sensing analysis is just in its early stage. There are still some problems to be solved in theoretical research and practical application, such as unclear photoelectric response mechanism, low intensity of electrochemiluminescence and many influencing factors of photocurrent change. A large number of systematic and comprehensive studies are needed to reveal the intrinsic mechanism of quantum dot-based photoelectric conversion. In addition, electron-hole recombination is easy to occur when simple quantum dots are excited by light, and the photoelectric conversion efficiency is not high. To improve the photoelectric property and biocompatibility of quantum dots by introducing inorganic nanomaterials or organic materials with matching energy levels, designing a range of sensitive photoelectrochemical sensors have become the focus of current reports in the literature.
Therefore, based on extensive literature review, the principles and advantages of quantum dots used in photoelectrochemical sensors are described in detail in this paper. The commonly used photoelectric composite materials of quantum dots and the methods of constructing sensing interfaces are summarized. The applications of quantum dots in photoelectrochemical sensing detection of metal ions, small molecule compounds and biological analysis are comprehensively reviewed. Finally, current challenges and future perspectives in this field are also discussed to promote new developing directions.

Key words： quantum dots composite photoelectric effect photoelectrochemical sensor

Received: 25 September 2022 Published: 25 September 2022 Online: 2022-09-26

CLC number:	O657.3
	O649.3
	O482.7

Fund:The National Natural Science Foundation of China (41977129), the Natural Science Foundation of Hunan Province(2022JJ90020), the Opening Fund of Key Laboratory of Chemical Biology and Traditional Chinese Medicine Research (Ministry of Education), Hunan Normal University (KLCBTCMR18-07).

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	WANG Qiong
	ZHANG Yi
	TANG Hao
	HU Yunchu
	WANG Wenlei

Cite this article:

WANG Qiong,ZHANG Yi,TANG Hao, et al. Recent Progress of Quantum Dots in Photoelectrochemical Sensors[J]. Materials Reports, 2022, 36(18): 20090134-8.

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http://www.mater-rep.com/EN/10.11896/cldb.20090134 OR http://www.mater-rep.com/EN/Y2022/V36/I18/20090134

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