| METALS AND METAL MATRIX COMPOSITES |
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| Research Progress in Metal-organic Frame Materials for Adsorptive Removal of Contamination in Wastewater |
| FU Qingshan, ZHANG Lei1, ZHANG Wei1, ISMAIL Pir-Muhammad1, CHEN Xuedan1, GONG Min1, HE Ping2, WANG Zubo2
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1 Materials Science and Engineering College, Sichuan University of Science & Engineering, Sichuan 643000, China;
2 China Carbon Black Institute, Sichuan 643000, China |
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Abstract The depletion of clean water has become a major global crisis, of which main reason is the water pollution caused by various pollutants discharged into the water due to production, living activities or accidents. Therefore, the key to solve the crisis lies in wastewater treatment and regeneration. A variety of water treatment and regeneration methods have emerged, among which adsorption has become a widely used sewage treatment method owing to its high performance, simple operation and low cost.
Choice and application of eligible adsorbents determine the performance of an adsorption process. Traditional adsorbents used in water treatment, such as activated carbon, zeolite, natural clay and activated alumina, cannot meet the higher and higher requirements of wastewater treatment for kinds of pollutants with different properties in complex water environment. For this reason, the development and utilization of new adsorbents have become a research hotspot in the field of adsorption.
Metal?organic frame (MOF) materials, a type of compound formed by self?assembly between metal ions or metal clusters and organic ligands, has attracted increasing attention in the field of adsorption due to its huge specific surface area, high porosity and controllable pore structure. At present, the researches of MOF materials as adsorbents for water treatment mainly focus on: (1) adsorption performance of various MOF mate?rials for different contaminations to reveal the relevant adsorption rules; (2) modification of MOF or preparation of MOF composite materials to improve self?stability and adsorption performance or achieve selective adsorption; (3) fabrication of MOF?derived carbon adsorbents for application in harsh water environment or extreme water treatment conditions.
This review includes the researches related to single MOF materials, functionalized MOF materials, and MOF?derived carbon materials for the adsorptive removal of organic dyes, other organic pollutants and heavy metal ions in water. We review the different adsorptive capacities of va?rious MOF materials for kinds of contaminations in water, the diversified functionalization methods of MOF in order to boost adsorption perfor?mance and extent their application, and the exhibition of MOF?derived carbonaceous adsorbents in water treatment. Finally, we also point out the current main issues of MOF adsorbents in water treatment, and put forward some ideas to solve these problems.
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Published: 25 June 2021
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| Fund:The work was supported by the National Natural Science Foundation Project of China (51902216), Sichuan Provincial Science and Technology Department Project (2018JY0493), Sichuan Provincial Department of Education Project (18ZA0351), Talent Introduction Fund of Sichuan University of Light and Chemical Technology(2017RCL27), Graduate Innovation Fund of Sichuan University of Light and Chemical Technology(y2019024). |
| About author:: Qingshan Fu, professor, tutor of postgraduates, received his bachelor, master and doctoral degrees from Sichuan University in 2004, 2007 and 2011, respectively, and has served at Sichuan University of Science & Engineering since 2012. Then he worked on MOF materials research at the University of Liverpool, and conducted postdoctoral work in China Carbon Black Institute. Currently, he is mainly engaged in researches on related materials for wastewater treatment and new energy devices. It mainly includes metal-organic framework materials, carbon nanomaterials, and electrospun membrane materials. Lei Zhang received his bachelor’s degree in Sichuan University of Science & Engineering in 2017, and then joined the new carbon material with Professor Qingshan Fu’s research group. Currently, he is mainly engaged in the synthesis and preparation of metal organic framework material (MOF), which is used for the research of adsorption and removal of harmful substances in wastewater. |
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2021, Vol. 35 
