磁响应吸油材料的研究进展

doi:10.11896/cldb.18110136

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Abstract The oil pollutants in the ocean mainly are from oil recovery and blowout, oil leakage from transport ships and oil pipelines. With the rapid growth of global energy consumption, oil extraction and transportation have become frequent. However, the problem derived from this process is also serious. It is estimated that the annual oil spill in the world is as high as 400 000 t on average.
Large-scale marine oil spill treatments mainly include three methods: physical treatment, chemical treatment and biological treatment. Among them, chemical methods such as in-situ combustion and dispersant degradation are high costs and secondary damage to the environment. Biolo-gical methods such as microbial decomposition are very demanding on natural conditions. Physical methods such as using mechanical devices (skimmers or booms ) require to input energy or high pressure operation. None of these methods adequately meet the requirements for oil spill treatment.
Recently, a method for oil-water separation which used a magnetically modified superhydrophobic/lipophilic oil absorption material has been originally proposed. These materials are mainly composed of clay (silica), zeolite, activated carbon, carbon nanotubes, polymers, wool and straw. The magnetic response of the material are imparted by embedding or coating of the ferric oxide nanoparticles. Adsorbent materials which have high porosity, high specific surface area and rich pore structure can be designed and prepare magnetic oil absorption materials that are superior to traditional methods in oil removing, oil recovery and operating cost after magnetic particles modified. The magnetically oil absorption materials based on polymers are the most widely studied. The polymer sponge coated with magnetic nanoparticles can absorb up to 50 g/g, and all have an efficiency close to 95%. Other materials have also been reported. These magnetic oil absorption materials have three major characteristics: (1) high oil absorption efficiency and stable oil absorption; (2) oil-locking performs well and adsorbed oil is difficult to desorb; (3) easy to recycle and reuse.
This review explains the mechanism of oil absorption and magnetic modification, analyzing oil absorption tests and recycling experiments of typical magnetic oil absorption materials, advantages and disadvantages of various types of oil absorption materials in the process of oil spill are poin-ted out. Among them, fly ash zeolites which are magnetically modified have been specially proposed. Latest research in the field of solid waste resources is put forward. Hope to be significant for relevant fields in China.

Key words： oil spill magnetic oil-water separation oil absorption materials recycle solid waste resources

Published: 30 September 2019

CLC number:

TE992.4

Fund:This work was financially supported by the National Natural Science Foundation of China (21766013), the National College Students’ Innovation and Entrepreneurship Training Program (201710674111), the Analysis and Testing Foundation of Kunming University of Science and Technology (2016T20070105).

About author:: Guangbing Liang received his B.S. degree in applied chemistry from Northeast Petroleum University in 2018. He is currently pursuing his M.E. in Chemical Engineering at Kunming University of Science and Technology under the supervision of Dr. Yanhong Li. His research has focused on magnetic oil-water separation materials.
Yanhong Li received his B.E. in chemical engineering from Xinyang Normal University in 2004 and received his M.S. in chemical engineering from Taiyuan University of Technology in 2007 and is currently pursuing his Ph.D. at Taiyuan University of Technology. His research has focused on energy and chemical engineering, such as biomass, coal and petroleum.

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	LIANG Guangbing
	LI Yanhong
	ZHANG Yuanqin
	ZI Changyu
	ZHAO Wenbo
	ZHANG Dengfeng

Cite this article:

LIANG Guangbing,LI Yanhong,ZHANG Yuanqin, et al. Progress on Magnetically Responsive Oil Absorption Materials[J]. Materials Reports, 2019, 33(23): 3999-4007.

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http://www.mater-rep.com/EN/10.11896/cldb.18110136 OR http://www.mater-rep.com/EN/Y2019/V33/I23/3999

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