D-氨基酸增强型杀菌剂对三种金属材料腐蚀行为的影响

doi:10.11896/cldb.23090099

Abstract
Figure/Table
References
Related Citation (2)

Download:

Full Text ( PDF ) (4341KB)
Export: BibTeX | EndNote (RIS)

Abstract The effects of D-amino acid enhanced compound bactericide on corrosion resistance behavior and mechanism of 45# carbon steel, 316L stainless steel and H62 brass in sulfate reducing bacteria (SRB) + iron oxidizing bacteria (IOB) were studied by biological culture technology, bactericidal process evaluation, weight loss experiment, electrochemical test and surface analysis. The results showed that the corrosion depth of different metals a year without bactericide was as follows, 45# carbon steel (0.104 2 mm/a) ＞H62 brass (0.045 6 mm/a) ＞ 316L stainless steel (0.007 3 mm/a). Because the SRB and IOB in the mixed bacteria have a synergistic effect to accelerate the corrosion of metal mate-rials. After adding the bactericide, the bactericidal rate of SRB and IOB in the mixed bacteria exceeded 99% and 90%, respectively, the polarization curves of the three metals all shifted to the left, the i_corrdecreased in a varying degree, the corrosion rate reduced significantly, and the depth and number of pitting pits decreased significantly. Moreover, the content of P and S in microbial metabolites decreased significantly, it indicated that the number of viable bacteria decreased sharply. With or without bactericide, 316L stainless steel has the best corrosion resistance due to the easy formation of chromium oxide passivation film on the surface, and H62 brass has good corrosion resistance due to Cu²⁺bactericidal effect. The tetrakis hydroxymethyl phosphonium sulphate (THPS) in the compound bactericide can change the properties of cellular enzymes and proteins to cause the death of bacteria, meanwhile D-amino acids can decompose the biofilm on the surface of the metal, which can change the bacteria from the hard-to-kill fixed state to the easy-to-kill floating state to improve the bactericidal effect, and also avoid the formation of high concentrations of extracellular polymer EPS, thereby reduce the corrosion rate of the metal.

Key words： D-amino acids bactericide mixed bacteria biofilms metallic corrosion resistance

Published: 25 October 2024 Online: 2024-11-05

CLC number:

TG172.4

Fund:National Natural Science Foundation of China (51974245, 21808182), Shaanxi Provincial Key R & D Program (2020GY-234), Xi’an Key Laboratory of High Performance Oil and Gas Field Materials, School of Materials Science and Engineering, Xi’an Shiyou University, Xi’an Shiyou University ‘Materials Science and Engineering’ Provincial Advantageous Discipline Funding Project (YS37020203), Xi’an Shiyou University Postgraduate Innovation and Practical Ability Training Project (YCS22213138).

	Service
	E-mail this article
	Add to my bookshelf
	Add to citation manager
	E-mail Alert
	RSS
	Articles by authors
	XU Congmin
	LI Xueli
	ZHU Wensheng
	ZHU Shidong
	YANG Xing
	GAO Haoran
	SUN Shuwen

Cite this article:

XU Congmin,LI Xueli,ZHU Wensheng, et al. Effect of D-amino Acid Enhanced Bactericide on Corrosion Behavior of Three Metal Materials[J]. Materials Reports, 2024, 38(20): 23090099-6.

URL:

http://www.mater-rep.com/EN/10.11896/cldb.23090099 OR http://www.mater-rep.com/EN/Y2024/V38/I20/23090099

1 Little B J, Blackwood D J, Hinks J, et al. Corrosion Science, 2020, 170, 108641.
2 Liu L, Fu Q, Peng C, et al. Journal of Pipeline Systems Engineering and Practice, 2022, 13(3), 04022014.
3 He Y J, Zhang T S, Wang H T, et al. Chinese Journal of Corrosion and Protection, 2021, 41(6), 748 (in Chinese).
何勇君, 张天遂, 王海涛, 等. 中国腐蚀与防护学报, 2021, 41(6), 748.
4 Taghavi K S, Rasekh B, Yazdian F, et al. International Journal of Environmental Science and Technology, 2021, 18, 195.
5 Wei B X, Xu J, Gao L Q, et al. Surface Technology, 2021, 50(3), 30 (in Chinese).
韦博鑫, 许进, 高立群, 等. 表面技术, 2021, 50(3), 30.
6 Wan H, Zhang T, Wang J, et al. Bioelectrochemistry, 2023, 150, 108367.
7 Wang Z Q, Xu W C, Zhou Z Y, et al. Surface Technology, 2020, 49(7), 245 (in Chinese).
王正泉, 徐玮辰, 周子扬, 等. 表面技术, 2020, 49(7), 245.
8 Lovley D R. Bioresource Technology, 2022, 345, 126553.
9 Qian H C, Chang W W, Cui T Y, et al. Corrosion Science, 2021, 191, 109751.
10 Koegler F, Hartmann F S F, Schulze-Makuch D, et al. International Biodeterioration & Biodegradation, 2021, 157(6), 105158.
11 Bai Y L, Shen G L, Qin Q Y, et al. China Journal of Corrosion and Protection, 2021, 41(1), 60 (in Chinese).
白云龙, 沈国良, 覃清钰, 等. 中国腐蚀与防护学报, 2021, 41(1), 60.
12 Vaithiyanathan S, Chandrasekaran K, Barik R C. Biotechnology & Applied Microbiology, 2018, 8, 1.
13 Xu J, Jia R, Yang D Q, et al. Journal of Materials Science & Technology, 2018, 35(1), 109.
14 Jia R, Yang D Q, Hasrizal B A R, et al. International Biodeterioration & Biodegradation, 2017, 125, 116.
15 Liu H W, Fu C Y, Gu T Y, et al. Corrosion Science, 2015, 100, 484.
16 Xu C M, Luo L H, Wang W Y, et al. Journal of Chinese Society for Corrosion and protection, 2020, 40(1), 63 (in Chinese).
胥聪敏, 罗立辉, 王文渊, 等. 中国腐蚀与防护学报, 2020, 40(1), 63.
17 Guo N, Mao X M, Hui X R, et al. Chinese Journal of Corrosion and Protection, 2022, 42(5), 743 (in Chinese).
郭娜, 毛晓敏, 惠芯蕊, 等. 中国腐蚀与防护学报, 2022, 42(5), 743.
18 Xu C, Gao H, Zhu W, et al. Materials, 2021, 14(22), 6981.
19 Xu C M, Gao H R, Zhu W S, et al. Materials Reports, 2023, 37(1), 243 (in Chinese).
胥聪敏, 高豪然, 朱文胜, 等. 材料导报, 2023, 37(1), 243.
20 Li Y. Pretreatment technology and properties of electroless nickel-phosphorus plating on SiCp/Al matrix composites. Master’s Thesis, Xi’an Technological University, China, 2022 (in Chinese).
李岳. SiCp/Al基复合材料化学镀镍-磷镀层的前处理工艺与性能研究. 硕士学位论文, 西安工业大学, 2022.
21 Xu C M, Wang W Y, Liu L, et al. Natural Gas Industry, 2021, 41(2), 160 (in Chinese).
胥聪敏, 王文渊, 刘利, 等. 天然气工业, 2021, 41(2), 160.