POLYMERS AND POLYMER MATRIX COMPOSITES |
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Recent Progresses in Photocatalytic and Electrocatalytic Upcycling of Plastic Wastes to High Value-added Chemicals |
LIU Ruiqi, SUN Shanfu*, CHENG Pengfei, WANG Yinglin, HAO Xidong
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School of Aerospace Science and Technology, Xidian University, Xi’an 710126, China |
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Abstract The recycling and utilization ofplastic wastes is one of the effective ways to reduce environmental pollution and resource waste. Compared to the traditional mechanical cycle and chemical cycle recycling, the newly emerging photocatalytic and electrocatalytic waste plastic upcycling high value-added chemical technologies have aroused widespread attention due to their mild reaction conditions, high efficiency, and can use renewable energy to drive the reactions. It is expected to realize the circumvention resources of fossil fuel and chemicals development, which is in line with the carbon peaking and carbon neutrality goals. Herein, the latest research progress on photocatalytic and electrocatalytic upcycling of high value-added chemicals from waste plastics in recent years was reviewed, with emphasis on the effects of catalyst types on product types and yields, as well as the reaction paths and mechanisms of different catalysts. Ultimately, in view of the problems with these current technologies, points out the main research directions in future, including the development of efficient photo-/electrocatalytic catalysts to improve the selectivity and yield of high value-added products, theoretical simulation combined with in-situ characterization technologies to explore the mechanisms of catalytic reactions, and the development of efficient catalytic reaction equipment.
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Published: 25 October 2024
Online: 2024-11-05
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Fund:National Natural Science Foundation of China (22205169). |
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