二维材料用于电化学法制备过氧化氢的研究进展

doi:10.11896/cldb.22120169

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Abstract The electrochemical production of hydrogen peroxide via the two-electron oxygen reduction reaction (ORR) is a green, mild, and on-demand strategy. The key to this process is highly active, selective, and stable electrocatalysts. Noble metal catalysts are the most effective catalysts for the electrochemical production of hydrogen peroxide due to their unique physical and chemical properties. However, low-cost catalysts are essential for achieving the large-scale production of hydrogen peroxide. Therefore, reducing the dosage of precious metals or finding affor-dable and readily available alternatives has been a topic of considerable research interest in recent years. Numerous non-precious metals or non-metallic materials have been used in oxygen reduction electrocatalysts, some of which have comparable or even superior electrochemical perfor-mances compared to noble metal catalysts. Furthermore, the band structures and surface structures of two-dimensional materials are easier to adjust than those of bulk materials. Two-dimensional materials exhibit faster electron transportation, achieve higher atomic utilization, and possess more exposed active sites. This review discusses the reaction mechanisms of the two-electron ORR for hydrogen peroxide production based on reported experimental results and theoretical calculations, and collates recent reports on the use of graphene, two-dimensional transition metal chalcogenide compounds, two-dimensional MOFs/COFs, g-C₃N₄, and MXenes as electrocatalysts for the ORR. Finally, the remaining challenges of the application of two-dimensional materials as oxygen reduction electrocatalysts are briefly summarized.

Key words： electrocatalysis two-electron oxygen reduction hydrogen peroxide two-dimensional materials

Published: 25 June 2024 Online: 2024-06-25

CLC number:

O64

Fund:Youth Innovation Promotion Association of the Chinese Academy of Sciences (2019374) and the Natural Science Foundation of Chongqing (cstc2021jcyj-msxmX0923).

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	Articles by authors
	SHENG Xiong
	LI Bangxing
	LU Shun
	LU Wenqiang
	LI Xiaofeng
	KANG Shuai

Cite this article:

SHENG Xiong,LI Bangxing,LU Shun, et al. Research Progress on Electrochemically Producing Hydrogen Peroxide Using Two-dimensional Materials as Catalysts[J]. Materials Reports, 2024, 38(11): 22120169-13.

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http://www.mater-rep.com/EN/10.11896/cldb.22120169 OR http://www.mater-rep.com/EN/Y2024/V38/I11/22120169

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