锂离子电池用纳米碳材料研究进展

doi:10.11896/cldb.21050286

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Abstract As one of the most promising energy storage devices, lithium-ion batteries have been widely used in portable electronic devices. However, the inadequate energy density and power density, poor durability and high cost, which are resulted from using traditional electrode materials, limit the large-scale applications of lithium-ion batteries in electric vehicles. The development of carbon nanomaterials provides an opportunity for the new energy storage materials applied in lithium-ion batteries. Nanocarbons have many unique characteristics, including unique morphology and microstructure, high specific surface area, low diffusion distance, high electronic and ionic conductivity, controllable synthesis and doping, etc. Therefore, nanocarbons have great application prospects in the field of lithium-ion batteries with high reversible capacity, high power density, good cycle stability and high safety.
However, nanocarbons as electrode materials exhibit low initial Coulombic efficiency and large voltage hysteresis during charging/discharging. Moreover, the electrochemical performance of nanocarbons is dependent on their morphology and microstructure. The following strategies are proposed to solve these problems: (Ⅰ) improving the electrochemical performance by adjusting the morphology and microstructure of nanocarbons; (Ⅱ) improving electrochemical performance by doping heteroatoms into nanocarbons; (Ⅲ) combining nanocarbons with other materials to form carbon-based composites for high-performance lithium storage.
The recent progress of nanocarbon materials in lithium-ion batteries, typically represented by fullerene, graphene, carbon nanotubes and po-rous carbon is reviewed in this paper. The influence of nano-size and morphology on the electrochemical performance of nanocarbons is also summarized. The synthesis of nano-carbon, lithium-ion battery performance and electrode reaction mechanism are emphasized. The purpose of this paper is to summarize the recent progress of carbon nanomaterials in the lithium-ion batteries and their key fundamental problems to be solved in the future.

Key words： nanocarbon lithium-ion battery fullerene graphene carbon nanotube porous carbon

Published: Online: 2022-10-26

CLC number:

TM911

Fund:National Natural Science Foundation of China (52072342,51677170), Zhejiang Natural Science Foundation of China (LY19E010007) and Open Fund of Fujian Provincial Key Laboratory of Functional Materials and Applications (fma2020003).

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	Articles by authors
	ZHANG Bailun
	WANG Kai
	LI Jiahui
	ZHONG Haichang
	ZHANG Wenkui
	ZHANG Wenxian
	LIANG Chu

Cite this article:

ZHANG Bailun,WANG Kai,LI Jiahui, et al. Progress in Carbon Nanomaterials for Lithium-ion Batteries[J]. Materials Reports, 2022, 36(20): 21050286-13.

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http://www.mater-rep.com/EN/10.11896/cldb.21050286 OR http://www.mater-rep.com/EN/Y2022/V36/I20/21050286

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