| INORGANIC MATERIALS AND CERAMIC MATRIX COMPOSITES |
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| Research Advances on Modified Titanium Dioxide for Photogenerated Cathodic Protection |
| LONG Wujian1,2, MING Gaolin1,2, DONG Biqin1,2, FU Xianzhu3, LUO Jingli3, SHI Shi1,2,*
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1 College of Civil and Transportation Engineering, Shenzhen University, Shenzhen 518060, Guangdong, China
2 Guangdong Provincial Key Laboratory of Durability for Marine Civil Engineering, Shenzhen 518060, Guangdong, China
3 College of Materials Science and Engineering, Shenzhen University, Shenzhen 518060, Guangdong, China |
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Abstract The extensive application of metal materials has greatly promoted the social progress. However, the high-frequency metal corrosion causes huge losses and harm to human life and safety, which triggers a series of ecological problems as well. Generally, corrosion protection measures have been carried out, such as materials selection, coating, corrosion inhibitor and electrochemical protection. Cathodic protection, one of the electrochemical protection techniques, has been widely used in metal corrosion protection, yet there are some limitations for traditional cathodic protection technologies. As for traditional cathodic protection technologies, current-impressed cathodic protection requires regular maintenance, monitoring and complicated devices, while sacrificial anode cathodic protection with low output needs replacing anode metal regularly. In the past two decades, photogenerated cathodic protection, a novel approach of cathodic protection technology, has attracted a great deal of attention and confirmed to be truly efficient and eco-friendly, in which semiconductors serve as photoelectric center to transform solar radiation into electricity. The photoelectric conversion efficiency of semiconductor materials is focused on, as well as the ability of photogenerated electrons transferring and enriching onto the protected metal surface. TiO2 is a kind of photoelectric pollution-free semiconductor material, which shows good stability and excellent photocorrosion resistance. There are broad application prospects for TiO2 in the fields of photocatalytic activity, photoelectric conversion, photogenerated cathodic protection and others. However, the characteristics of wide band gap, poor photoresponse ability, high photocarrier recombination velocity and inefficient photoelectric conversion lead to insufficiency in offering sustained protection. Therefore, breaking through bottlenecks of TiO2 application in photogenerated cathodic protection by effective modification has recently received significant attention. Different modification methods for TiO2 to improve photoelectric conversion efficiency have been studied carefully. A great breakthrough in the substantiation of photogenerated cathodic protection in darkness has been performed.
This review, proceeding from the mechanism of photogenerated cathodic protection, systematically introduces modification methods including metal deposition, ion doping, semiconductor compounding (g-C3N4, Bi2S3, graphene, etc.) and quantum dots sensitization. Advances of different modification methods of TiO2 in improving efficiency of photoelectric performance and photogenerated cathodic protection are emphatically discussed. The research advances and achievements of the author's team on photocatalytic materials and corrosion protection are reviewed. In addition, the feasibility of cathodic protection for reinforcement is demonstrated. Finally, future research direction and research emphases of photogenerated cathodic protection are proposed. This review provides new approaches for the wide application of modified TiO2 in photogenerated cathodic protection in a sustainable way.
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Published: 10 August 2022
Online: 2022-08-15
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| Fund:National Natural Science Foundation of China (U2006223, 51778368) and Science and Technology Project of Shen-zhen, China (JCYJ20180305124844894, JCYJ20190808151011502). |
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2022, Vol. 36 
