| ELECTROCHEMICAL ENERGY MATERIALS AND DEVICES |
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| Research Advances of Metal-based Phosphide Nanomaterials Toward Electrocatalytic Applications |
| LIU Hui1, YANG Niuwa1,2, MA Mengyuan1,2, TIAN Shaonan1,*, ZHANG Yu1, YANG Jun1,2,*
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1 State Key Laboratory of Mesoscience and Engineering, Institute of Process Engineering, Chinese Academy of Sciences, Beijing 100190, China
2 Center of Materials Science and Optoelectronics Engineering, University of Chinese Academy of Sciences, Beijing 100049, China |
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Abstract Nanometer sized metal phosphides and their nanocomposites with noble metals have unique physical/chemical properties that have been found wide applications in electrocatalysis. For instance, in methanol oxidation reaction, the shift of electron clouds from noble metals, e.g. Pt and Pd, to the phosphor (P) due to larger electronegativity of the latter would enhance thetolerance of noble metals for the CO-like interme-diates produced during methanol oxidation. Also, in hydrogen evolution reaction (HER) of electrocatalytic water splitting, the P element in the phosphide-based nanocomposites could strengthen the H+ adsorption by serving as proton acceptor, thus promoting the HER. In addition, in oxygen evolution reaction (OER), the metal phosphides could be easily transformed into metal oxides/hydroxides for forming metal phosphide-metal oxide/hydroxide interfaces that is capable to boost the OER. It is well known that the catalytic performance of a catalyst strongly depends on its structure, components and their interactions as well as the electronic configuration of the active sites. In this context, rational regulation of the above-mentioned properties of metal phosphide-based nanocomposites is of necessity to improve their electrocatalytic performance. It is noteworthy that the materials in this review include metal phosphides and their nanocomposites with different nobles. We would firstly introduce the synthesis and characterization of metal phosphide-based nanocomposites, and subsequently, we focus on reviewing recent advances and challenges in making use of the lattice strain effect and electronic coupling effect to boost the performance of metal phosphide-based nanocomposites in typical electrochemical reactions. Eventually, regarding further improvement in elecrtocatalytic performance, we make some perspectives on the future synthetic strategies and development of the metal phosphide-based nanocomposites.
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Published: 25 April 2024
Online: 2024-04-28
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| Fund:National Natural Science Foundation of China (22075290, 22272179) and Beijing Natural Science Foundation (Z200012). |
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2024, Vol. 38 
