METALS AND METAL MATRIX COMPOSITES |
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Effect of Reaction Time of One-step on Corrosion Resistance of Superhydrophobic Coatings on AZ91 Magnesium Alloys |
LI Shaopeng, WANG Defang, XIE Wenling*, LI Xiulan, Li Xuan
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College of Mechanical Engineering, Sichuan University of Science and Engineering, Zigong 643000, Sichuan, China |
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Abstract One-step method combined hydrothermal etching and modification using stearic acid ethanol and zinc sulfate solution was used to prepare superhydrophobic coatings on the AZ91 magnesium alloys. The effect of reaction times of the one-step method on hydrophobicity and corrosion resistance of superhydrophobic coatings was studied. The phase composition and microstructure of coatings were analyzed by X-ray photoelectron diffractometer (XRD), Fourier transform infrared ray (FTIR), scanning electron microscope (SEM) and EDS spectrum. And the hydrophobicity and corrosion resistance were characterized by contact angle and polarization curve. With the increase of reaction time, the contact angles of the coatings first increased and then decreased. The coating prepared with 7 h of action time had the maximum contact angles of 154.2°, which was a superhydrophobic coating, and the coated sample had the lowest corrosion current density and the biggest impedance, which was 3 orders of magnitude lower and 5 orders of magnitude higher than those of uncoated magnesium alloy matrix, respectively. So, the corrosion resistance of the magnesium alloy was significantly improved.
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Published: 25 September 2023
Online: 2023-09-18
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Fund:Key Laboratory Project of Process Equipment and Control Engineering in Sichuan Universities (GK202011) and College Students' Innovation and Entrepreneurship Project (cx2020176). |
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1 Kubásek J, Minárik P, Hosová K, et al. Journal of Alloys and Compounds, 2021, 877, 160089. 2 Feliu Jr S, Galván J C, Pardo A, et al. The Open Corrosion Journal, 2010, 3(1), 80. 3 Liu S, Li Z, Yu Q, et al. Chemical Engineering Journal, 2021, 424, 130551. 4 Zou Y, Wang Y, Xu S, et al. Chemical Engineering Journal, 2019, 362, 638. 5 Wang Z, Su Y, Li Q, et al. Materials Characterization, 2015, 99, 200. 6 Wang L, Yang J, Zhu Y, et al. Materials Letters, 2016, 171, 297. 7 Zheng T, Hu Y, Zhang Y, et al. Journal of Colloid and Interface Science, 2017, 505, 87. 8 Wan H, Hu X. Materials Letters, 2016, 174, 209. 9 Li J, Liu Q, Wang Y, et al. Journal of the Electrochemical Society, 2016, 163(5), C213. 10 Li Y, Dai S, John J, et al. ACS Applied Materials & Interfaces, 2013, 5(21), 11066. 11 Guo Z, Liu W, Su B L. Journal of Colloid and Interface Science, 2011, 353(2), 335. 12 Qian H C, Li H Y, Zhang D W. Surface Technology, 2015 (3), 15 (in Chinese). 钱鸿昌, 李海扬, 张达威. 表面技术, 2015 (3), 15. 13 Çamurlu H E, Mathur S, Arslan O, et al. Ceramics International, 2016, 42(5), 6312. 14 Gunasekaran S, Natarajan R K, Kala A. Spectrochimica Acta Part A: Molecular and Biomolecular Spectroscopy, 2007, 68(2), 323. 15 Ng W F, Wong M H, Cheng F T. Surface and Coatings Technology, 2010, 204(11), 1823. 16 Sun X D, Liu G, Li L Y. Chinese Journal of Materials Research, 2015, 29(7), 523 (in Chinese). 孙小东, 刘刚, 李龙阳. 材料研究学报, 2015, 29(7), 523. 17 Sundaraganesan N, Joshua B D. Spectrochimica Acta Part A: Molecular and Biomolecular Spectroscopy, 2007, 68(3), 771. 18 Xue H X, Li J P, Xu Z Q, et al. Journal of Fuel Chemistry and Techno-logy, 2009, 37(6), 747 (in Chinese). 薛海霞, 李军平, 许振芹, 等. 燃料化学学报, 2009, 37(6), 747. 19 Li H Y, Tang Y X, Xu Z Q. Chinese Journal of Lasers, 2006, 33(1), 116 (in Chinese). 李海元, 唐永兴. 中国激光, 2006, 33(1), 116. 20 Zhang Y, Zhu H, Zhuang C, et al. Materials Chemistry and Physics, 2016, 179, 80. 21 Li M, Wang L, Li D, et al. Carbohydrate Polymers, 2014, 102, 136. 22 Wang Q, Han S L, Guo F, et al. Journal of Fuel Chemistry and Techno-logy, 2019, (3), 340 (in Chinese). 王茜, 韩素立, 郭峰, 等. 摩擦学学报, 2019 (3), 340. 23 Whyman G, Bormashenko E, Stein T. Chemical Physics Letters, 2008, 450(4-6), 355. 24 Fini M H, Amadeh A. Transactions of Nonferrous Metals Society of China, 2013, 23(10), 2914. 25 Yu D, Tian J. Colloids and Surfaces A: Physicochemical and Engineering Aspects, 2014, 445, 75. 26 Ouyang X, Qiu X, Lou H, et al. Industrial & Engineering Chemistry Research, 2006, 45(16), 5716. 27 Zhang K, Wen B W, Tan Y. Corrosion Science and Protection Technology, 2018, 30(4), 441 (in Chinese). 张凯, 文邦伟, 谭勇. 腐蚀科学与防护技术, 2018, 30(4), 441. 28 Floyd F L, Avudaiappan S, Gibson J, et al. Progress in Organic Coa-tings, 2009, 66(1), 8. 29 Chu J H, Tong L B, Jiang Z H. Surface Technology, 2019, 48(3), 62 (in Chinese). 楚景慧, 佟立波, 江忠浩. 表面技术, 2019, 48(3), 62. 30 Liu Y, Yin X, Zhang J, et al. Electrochimica Acta, 2014, 125, 395. 31 Zhong Y, Hu J, Zhang Y, et al. Applied Surface Science, 2018, 427, 1193. 32 Zhao H, Cai S, Ding Z, et al. RSC Advances, 2015, 5(31), 24586. 33 Ranganatha S, Venkatesha T V, Vathsala K. Applied Surface Science, 2010, 256(24), 7377. 34 Zhao B F, Zou D N, Tong L B. Surface Technology, 2021, 50(10), 322 (in Chinese). 赵碧芳, 邹德宁, 佟立波. 表面技术, 2021, 50(10), 322. 35 López-Ortega A, Bayón R, Arana J L. Surface and Coatings Technology, 2018, 349, 1083. |
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