硼/磷掺杂电解水析氢金属催化剂的研究现状与进展

doi:10.11896/cldb.22080121

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Abstract Hydrogenhas higher energy density with low-carbon, and is regarded as one of green energy technology for China ‘Double Carbon' plan. Hydrogen production by water electrolysis is called Green Hydrogen, which is an important hydrogen source for fuel cells. At present, precious metal catalyst is mainly used in hydrogen evolution reaction. Its high price has prevented the large-scale application of electrolytic water. Therefore, it is extremely urgent to develop low-cost catalysts. In this paper, non-precious metal catalysts, B doped catalysts, P doped catalysts and B/P co-doped catalysts for the hydrogen evolution are reviewed. The main role of B element doping in metal catalysts can increase the electron defects, the electrochemical surface area, and decrease the reaction resistance to improve the catalytic activity of hydrogen evolution. Doping P element facilitates the formation of intermediate H_ads, and effectively improves the catalytic kinetics of the hydrogen evolution. B/P co-doped catalysts show better catalytic activity even than B doping and P doping non-noble metal catalysts due to the synergistic effect between them and mental catalyst. The reaction mechanism of B doping and P doping non-noble metal catalysts are discussed. Finally, the prospect of B/P co-doped catalysts for the hydrogen evolution is looked forward.

Key words： water electrolysis HER electrocatalysts B/P co-doped catalysts

Published: Online: 2023-09-06

CLC number:

TK91

Fund:National Natural Science Foundation of China(21606115), Jiangsu Science and Technology Project(BE2020759), Jiangsu Province ordinary university natural sciences research project(23KJA480001), Xuzhou Science and Technology Project(KC20195), Postgraduate Research and Practice Innovation Project of Jiangsu Normal University (2021XKT1225, 2022XKT1324).

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	Articles by authors
	ZHUANG Mingxing
	KA GAI·Suoyintu
	FU Wenying
	SI Si
	YU Tianyu
	YANG Jundong
	ZHANG Jian
	LIANG Yuxin
	ZHAO Xinsheng
	WEI Yongsheng

Cite this article:

ZHUANG Mingxing,KA GAI·Suoyintu,FU Wenying, et al. Progress of Metal Catalysts Doping with Boron, Phosphorus Elements for Hydrogen Evolution Reaction in Water Electrolysis[J]. Materials Reports, 2023, 37(S1): 22080121-11.

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http://www.mater-rep.com/EN/10.11896/cldb.22080121 OR http://www.mater-rep.com/EN/Y2023/V37/IS1/22080121

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