碳基材料构建电化学传感器实现苯二酚异构体的超敏精准检测:综述

doi:10.11896/cldb.21080175

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Abstract Dihydroxybenzene isomers are common organic contaminants, including hydroquinone, catechol and resorcinol, which behave similar structures and physicochemical properties and often coexist in water. The isomers are widely utilized in industry as raw materials or interme-diates; however, they are highly toxic, carcinogenic and refractory. The resulting phenol-containing wastewater poses a major threat to environment and people health. Therefore, it is of critical significance to efficiently and accurately determine dihydroxybenzene isomers.
Electrochemical sensors exhibit high sensitivity, ultralow limits of detection (LOD), wide linear range, ease of operation and low cost, and they have been widely utilized in the sensing of contaminants such as heavy metals ions and phenols. Due to high conductivity, large specific-surface area, and good chemical stability, carbon-based nanomaterials can effectively promote the adsorption, mass transfer and electron transfer process, providing a good basis to implement the simultaneous detection of isomers. Furthermore, surface functionalization, doping and compounding of other nanomaterials can regulate the composition and structure of carbon-based materials, which can further facilitate their sensing performance.
This review briefly introduces the environmental hazards of dihydroxybenzene isomers and its corresponding detection methods. Then, we elaborate the research progress of simultaneous determination of dihydroxybenzene isomers by electrochemical sensors constructed of carbon-based materials, including electrochemical sensing performance, enhancement mechanism of performance, and the structure-activity relationship of electrochemical sensor constructed by carbon-based materials. And, the electrochemical oxidation pathways and reaction mechanisms of the three isomers are also discussed in detail. Finally, this review discusses the challenge of ultrasensitive and precise determination of isomers, for promoting the development of dihydroxybenzene sensors.

Key words： electrochemical sensor dihydroxybenzene isomer simultaneous determination carbon-based nanomaterial electrooxidation mechanism

Published: 10 March 2023 Online: 2023-03-14

CLC number:

X502

Fund:National Natural Science Foundation of China (21605110, 21972102), the Postgraduate Practice Innovation Program of Jiangsu Province (SJCX20_1101) and Entrepreneurship and Innovation Talents of Jiangsu Province.

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	RAO Qianghai
	HU Guangxuan
	ZHANG Chunmei
	YANG Hongbin
	HU Fangxin
	GUO Chunxian

Cite this article:

RAO Qianghai,HU Guangxuan,ZHANG Chunmei, et al. Electrochemical Sensor Construction of Carbon-based Materials for Ultrasensitive and Precise Determination of Dihydroxybenzene Isomers: a Review[J]. Materials Reports, 2023, 37(5): 21080175-17.

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http://www.mater-rep.com/EN/10.11896/cldb.21080175 OR http://www.mater-rep.com/EN/Y2023/V37/I5/21080175

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