氨硼烷水解制氢催化剂及其限域载体的形貌可控合成研究进展

doi:10.11896/cldb.20100246

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Abstract Ammonia borane (AB) has been considered as one of the most promising hydrogen storage materials due to its high hydrogen-storage content (19.6wt%) and stability under ordinary storage conditions. Catalyst is the core technology which can significantly increase the rate of dehydroge-nation of AB as ammonia borane is not easy to release hydrogen at room temperature without catalysts. However, metal catalyst particles are generally easy to be oxidized and agglomerate. In order to overcome this problem, a variety of supports have been chosen to disperse the catalyst on their surface or in their poresto suppress the agglomeration and oxidation. The overall morphology of the catalysts and their support greatly determines the specific surface area of the catalyst and distribution of catalyst active particles, thereby affecting the number and distribution of reactive sites, and has a significant impact on the catalytic activity and the service life of the catalyst. Therefore, this article has classified the overall morphology of catalyst and their support for hydrogen generation of ammonia borane and their support according to spatial dimensions, and haavesummarized their controllable synthesis methods and their catalytic effects on hydrogen generation of ammonia borane.

Key words： ammonia borane dehydrogenation catalyst morphology support

Published: 25 November 2022 Online: 2022-11-25

CLC number:

O643

Fund:Key Scientific Research Projects of Colleges and Universities of Henan Provincial Department of Education, China (21A150018).

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	LI Xiang
	ZHANG Jun

Cite this article:

LI Xiang,ZHANG Jun. Research Progress of Shape-controlled Synthesis of Catalysts and Domain Limited Supports for Ammonia Borane Dehydrogenation[J]. Materials Reports, 2022, 36(22): 20100246-9.

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http://www.mater-rep.com/EN/10.11896/cldb.20100246 OR http://www.mater-rep.com/EN/Y2022/V36/I22/20100246

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