应变工程对钙钛矿材料光电性质和稳定性的调制

doi:10.11896/cldb.20070095

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Abstract Halide perovskite materials have been one of the hottest topics in recent years due to their excellent optoelectronic properties. This upsurge was initially caused by perovskite solar cells, whose power conversion efficiency has exceeded 25% in just a few years. The halide perovskite materials also show huge potential in light-emitting devices, photodetectors, lasers and other optoelectronic devices. The further improvement of perovskite materials and device performance and stability is the key issue of researchers. Various strategies to improve the optoelectronic properties and stability of perovskite materials have also been proposed, such as film crystallization control, interface modification/defect passivation, component engineering, additive engineering, etc. In recent years, strain engineering has been found to be able to effectively improve the optoelectronic properties and device performance of halide perovskites, which provides a novel avenue for the optimization of device performance of perovskite materials. In this review, we start with the basic concept of stress and strain, then describe how to measure and evaluate the residual stress and strain of perovskite materials, as well as how residual stress and strain affect the device performance and the underlying mechanism, and summarize the strategy of applying stress and strain to perovskite material. Finally, the new research perspective of strain engineering to improve the device performance of perovskite materials is prospected.

Key words： halide perovskite stress-strain stability optoelectronic property

Published: 10 September 2022 Online: 2022-09-10

CLC number:

O472

Fund:National Natural Science Foundation of China (11674015, 21701009) and the Beijing Outstanding Young Scientists Projects (BJJWZYJH01201910005018).

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	WANG Chao
	YAN Zhengguang
	XIAO Jiawen

Cite this article:

WANG Chao,YAN Zhengguang,XIAO Jiawen. Modulating the Optoelectronic Properties and Stability of Perovskites by Strain Engineering[J]. Materials Reports, 2022, 36(17): 20070095-9.

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http://www.mater-rep.com/EN/10.11896/cldb.20070095 OR http://www.mater-rep.com/EN/Y2022/V36/I17/20070095

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