利用高压手段调控铁电材料结构与性能的研究进展

doi:10.11896/cldb.20110057

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Abstract Ferroelectric materials are an important class of functional materials with spontaneous polarization in a certain temperature range. Their spontaneous polarization can be reversed by an external electric field, and they have a wide application potential in electronic devices such as photovoltaic regulators and storage. At present, the development of ferroelectric materials for applications is severely constrained by their high resistance and low carrier concentration, so there is an urgent need to find a simple and effective method to optimize the ferroelectric properties and other physical properties of ferroelectric materials. Pressure control is an effective means to modulate the crystal structure and electronic configuration and regulate the physical properties of materials. Lower pressure can affect the balance between long-range Coulomb attraction and short-range electron repulsion in ferroelectrics, resulting in an obvious increase in short-range repulsion and a decrease in ferroelectricity. However, once the critical pressure is reached, the ferroelectricity begins to increase, and the ferroelectric phase transition occurs, thus changing the physical properties of materials. In recent years, the research on the structure and physical properties of ferroelectric materials regulated by pressure at home and abroad mainly focuses on exploring ferroelectric phase transition and other physical properties of materials caused by pressure, and exploring its internal influence mechanism.
As an important dimension to adjust and control the structure of ferroelectric crystals, pressure can replace doping to study the ferroelectric phase transition to some extent, and it can also stabilize the phase transition temperature. The improvement of dielectric and ferroelectric properties of materials due to domain wall change and de-aging process caused by high pressure can make the materials well applied in device equipment. Pressure can modulate the relaxation behavior of ferroelectric materials by affecting the polar nano-domains, and it can also change the magnetic sequence or symmetry of the magnetoelectric coupling material to change its ferroelectric properties. The synchronous enhancement of ferroelectric, electric transport and photoelectric properties can be realized in the high pressure phase of ferroelectric photovoltaic materials, relative to those in the low pressure phase, and the mechanism of ferroelectric photovoltaic can be further explored by means of high pressure.
This review summarizes the high pressure research progress of ferroelectric materials at home and abroad, discusses the structural evolution of ferroelectric materials under high pressure and its occurrence mechanism, and the influence of high pressure conditions on ferroelectric properties, dielectric properties, relaxation behavior, magnetoelectric coupling and photovoltaic properties of ferroelectric materials is introduced. These provide new ideas for the research and design of new high-performance ferroelectric materials using high pressure technology.

Key words： high pressure ferroelectric materials phase transition dielectric property

Published: 25 June 2022 Online: 2022-06-24

CLC number:

TN321

Fund:Shanghai “Science and Technology Innovation Action Plan” Natural Science Foundation Project (21ZR1421800).

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	Articles by authors
	GUAN Jiayi
	ZHANG Ganghua
	ZENG Tao
	BAI Jianfeng
	GU Weihua

Cite this article:

GUAN Jiayi,ZHANG Ganghua,ZENG Tao, et al. Research Progress in High Pressure on Tuning the Structural and Physical Properties of Ferroelectric Materials[J]. Materials Reports, 2022, 36(12): 20110057-8.

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http://www.mater-rep.com/EN/10.11896/cldb.20110057 OR http://www.mater-rep.com/EN/Y2022/V36/I12/20110057

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